superconductivity
State-of-the-art superconducting qubits rely on a limited set of thin-film materials. Expanding their materials palette can improve performance, extend operating regimes, and introduce new functionalities, but conventional thin-film fabrication hinders systematic exploration of new material combinations. Van der Waals (vdW) materials offer a highly modular crystalline platform that facilitates such exploration while enabling gate-tunability, higher-temperature operation, and compact qubit geometries. Yet it remains unknown whether a fully vdW superconducting qubit can support quantum coherence and what mechanisms dominate loss at both low and elevated temperatures in such a device. Here we demonstrate quantum-coherent merged-element transmons made entirely from vdW Josephson junctions. These first-generation, fully crystalline qubits achieve microsecond lifetimes in an ultra-compact footprint without external shunt capacitors. Energy relaxation measurements, together with microwave characterization of vdW capacitors, point to dielectric loss as the dominant relaxation channel up to hundreds of millikelvin. These results establish vdW materials as a viable platform for compact superconducting quantum devices.
Using determinant Quantum Monte Carlo, we investigate the interplay between doping, inter-layer tunneling and onsite Hund's coupling in stabilizing superconductivity (SC) in a two-orbital model for the bilayer Nickelate La3Ni2O7\text{La}_3\text{Ni}_2\text{O}_7. With realistic dispersion and for certain values of the interaction parameters, the auxiliary-field-decoupled fermion Hamiltonian has Kramers anti-unitary symmetries which guarantee the absence of a sign problem. The same anti-unitary symmetries can also be used to show there is a second instability towards (π,π)(\pi,\pi) exciton condensation in the strong interaction limit. We indicate the possible connection between this exciton order and the enigmatic density wave state observed in experiment, and clarify the decisive role played by the inter-layer tunneling in the competition between SC and exciton condensation. Finally, possible directions on how to enhance the SC transition temperature and stabilize the SC phase are also discussed.
Cuprate superconductors remain central to condensed matter physics due to their technological relevance and unconventional, incompletely understood electronic behavior. While the canonical phase diagram and low-energy models have been shaped largely by studies of underdoped and moderately doped cuprates, the overdoped regime has received comparatively limited this http URL, we track the evolution of the electronic structure from optimal to heavy overdoping in La2-xSrxCuO4(LSCO) using broadband optical spectroscopy across x=0.15-0.60. The measured spectral changes--including the redistribution of Zhang-Rice-related spectral weigh--are in qualitative agreement with determinant quantum Monte Carlo simulations of the three-orbital Emery model, which together indicate a pronounced reconstruction of the electronic structure beyond hole concentrations x>0.2. Guided by these observations, we propose a spontaneous checkerboard-type Zhang-Rice electronic configuration that captures the coexistence of itinerant and localized carriers characteristic of the heavily overdoped state. Our results refine the doping-dependent Zhang-Rice-based framework for cuprates, illuminate how correlations persist deep into the overdoped regime, and provide new constraints on microscopic mechanisms of high-temperature superconductivity, with broader implications for correlated transition-metal oxides.
We report the synthesis and physical properties of a polycrystalline, hexagonal boride YRu3_3B2_2. Our resistivity and heat capacity measurements indicate that YRu3_3B2_2 is a weakly coupled superconductor, with critical temperature TcT_c = 0.63 K and upper critical field μ0Hc2\mu_0 H_{c2} (0)=0.11 T. Density functional theory calculations, together with chemical-bonding analysis, reveal that the electronic states at and near the Fermi energy level are dominated by the Ru kagome sublattice.
In this work, we investigate the combined effects of Rashba spin-orbit coupling (RSOC) and non-Hermiticity on topological phase transitions in spinful p-wave Kitaev chains. While previous studies have separately examined non-Hermitian (NH) extensions of Kitaev chains and the effects of RSOC in Hermitian systems, the interplay between these two mechanisms remains largely unexplored. We analyze this interplay by considering two distinct types of complex on-site potentials: (i) a uniform gain/loss term and (ii) a complex quasiperiodic potential. We demonstrate that the impact of RSOC is highly model-dependent. In particular, RSOC does not affect the topological phase boundary in the Hermitian limit of the uniform gain/loss model (provided the spin-flip hopping is weaker than the pairing strength), but significantly alters the topological landscape in the NH regime. In contrast, for the quasiperiodic model, RSOC modifies the phase boundaries in both the Hermitian and non-Hermitian cases. Notably, we find that the combined interplay of non-Hermiticity and RSOC drives topological transitions at significantly lower potential strengths compared to the Hermitian limit. We derive analytical expressions for the topological phase transitions in both cases and validate our predictions through numerical calculations of energy spectra and real-space winding numbers. This work provides a comprehensive understanding of how non-Hermiticity and RSOC cooperatively reshape topological phase diagrams in one-dimensional superconducting systems.
We study superconductivity and superfluid weight of the two-dimensional α\alpha-T3\mathcal{T}_3 lattice with on-site asymmetries, hosting an isolated quasi-flat band with tunable bandwidth via a parameter α\alpha. Within a mean-field approximation of the attractive Hubbard model, we obtain the superconducting order parameters on the three inequivalent sublattices and show their strong dependence on α\alpha, interaction strength, and electron filling. At quasi-flat band filling, a superconducting gap opens and grows power-law fast with interaction strength, instead of the usual slow exponential growth, due to diverging density of states. We calculate the superfluid weight from linear response theory and study its band dispersion and geometric contributions. While the conventional part proportional to band derivatives is suppressed in the quasi-flat band regime, the contribution dominated by the quantum metric grows linearly for small interaction strength. We further demonstrate how tuning α\alpha enhances the quantum metric and thus the geometric superfluid weight especially near half-filling, while increasing on-site asymmetries increases the conventional contribution by broadening the quasi-flat band. We obtain the Berezinskii-Kosterlitz-Thouless transition temperature and demonstrate its strong dependence and enhancement with the parameter α\alpha. Our results establish a tunable flat band system, the α\alpha-T3\mathcal{T}_3 lattice model, as a candidate for tunable quantum geometry and superfluid weight and as a prototype of related behavior in tunable quantum materials.
Motivated by recent angle-resolved photoemission spectroscopy (ARPES) experiments, we analyze the temperature, frequency, and momentum dependence of the single-particle scattering rate in a model of the γ\gamma-band of Sr2_2RuO4_4 under strain, with particular emphasis on the behavior near the Lifshitz transition where the Fermi energy crosses a single Van Hove point. While the scattering rate is only moderately anisotropic at zero strain, we find that it becomes strongly anisotropic at the Lifshitz point. At the lowest energies, we recover the expected universal behavior: the scattering rate varies (ignoring logarithmic corrections) as τ1ω\tau^{-1}\sim \omega at the Van Hove point and as τ1ω3/2\tau^{-1}\sim \omega^{3/2} away from it. At higher energies, however, corrections of order ω2\omega^2 become important in both regimes. We show that the experimentally observed behavior τ1ωα\tau^{-1} \sim \omega^{\alpha} with α1.4(2)\alpha \approx 1.4(2) at the Van Hove point can be quantitatively explained by a superposition of linear and quadratic contributions to the scattering rate, which are comparable in magnitude at the intermediate energies probed by experiment, rather than in terms of a new universal power law. We further predict a distinctive anisotropy, strain dependence, and a non-monotonic frequency dependence of the scattering rate at a Lifshitz transition, all of which may be directly tested in experiments.
As quantum computing processors increase in size, there is growing interest in developing cryogenic electronics to overcome significant challenges to system scaling. Single flux-quantum (SFQ) circuits offer a promising alternative to remote, bulky, and power-hungry room temperature electronics. To meet the need for digital qubit control, readout, and co-processing, SFQ circuits must be adapted to operate at millikelvin temperatures near quantum processors. SEEQC's SFQuClass digital quantum management approach proximally places energy-efficient SFQ (ERSFQ) circuits and qubits in a multi-chip module. This enables extremely low power dissipation, compatible with a typical dilution cryostat's limited cooling power, while maintaining high processing speed and low error rates. We report on systematic testing from 4 K to 10 mK of a comprehensive set of ERSFQ cells, as well as more complex circuits such as programmable counters and demultiplexers used in digital qubit control. We compare the operating margins and error rates of these circuits and find that, at millikelvin, bias margins decrease and the center of the margins (i.e., the optimal bias current value) increases by ~15%, compared to 4.2 K. The margins can be restored by thermal annealing by reducing Josephson junction (JJ) critical current Ic. To provide guidance for how circuit parameters vary from 4.2 K to millikelvin, relevant analog process control monitors (PCMs) were tested in the temperature range of interest. The measured JJ critical current (of the PCM JJ arrays) increases by ~15% when decreasing temperature from 4.2 K to millikelvin, in good agreement with both theory and the empirically measured change in the center of bias margins for the tested digital circuits.
We present an advanced model for describing the readout power dependence of the resonance characteristics of a microwave SQUID multiplexer. Our model proves valid for SQUID screening parameters up to \beta_\mathrm{L}<1, hence covering the full range of practically relevant design parameters. We demonstrate that our model significantly improves agreement with experimental data compared to the existing models, thereby enabling optimization beyond the previously accessible parameter space. Moreover, our model supports non-sinusoidal current-phase relations of the rf-SQUID's Josephson junction, allowing, for the first time, for the modeling of devices based on Josephson tunnel junctions with inhomogeneous tunnel barriers. We show that the effects of such inhomogeneities are qualitatively similar to, yet distinct from, those of the screening parameter, making their inclusion essential for accurate characterization. Incorporating these effects yields great improved agreement with measurements, even at readout power conditions well beyond typical operating parameters.
Materials with a kagome sublattice have been heavily studied recently for their exotic electronic band structure, structural frustration, high-temperature charge order transitions, and unconventional electron-phonon coupling. In LaRu3Si2, it was proposed that electronic flat bands conspire with the characteristic phonon spectrum of the kagome lattice to drive enhanced superconductivity at Tc = 7 K. Here, we report bulk superconductivity in the structural analogue YRu3B2, which hosts a structurally pristine kagome lattice. We observe a superconducting transition at Tc = 0.7 K through magnetization, resistivity, and heat-capacity measurements in this novel kagome metal.
We report the effect of the \emph{ab}-plane magnetic field BB up to 8T8\,\mathrm{T} on the resistivity ρ(T)\rho(T) and fluctuation conductivity σ(T)\sigma'(T) in YBa2_2Cu3_3O7δ_{7-\delta} thin films. As expected, up to 2.5T\sim 2.5\,\mathrm{T} the magnetic field monotonously increases ρ\rho, the width of the resistive transition ΔTc\Delta T_c, and the coherence length along the cc axis, ξc(0)\xi_c(0), but decreases both TcT_c and the range of superconducting (SC) fluctuations Δfl\Delta _{\mathrm{fl}}. The fluctuation conductivity exhibits a crossover at characteristic temperature T0T_0 from the 3D Aslamazov--Larkin (AL) theory near TcT_c to the 2D fluctuation theory of Maki--Thompson (MT). However, at B=3TB = 3\,\mathrm{T}, the MT term is completely suppressed, and above T0T_0 σ(T)\sigma'(T) is unexpectedly described by the fluctuation contribution of 2D AL, suggesting the formation of a two-dimensional vortex lattice in the film under the action of a magnetic field. At the same time, ΔTfl\Delta T_{\mathrm{fl}} sharply increases by a factor of about 7, and ξc(0)\xi_c(0) demonstrates a very unusual dependence on TcT_c when BB increases above 3T3\,\mathrm{T}. Our results demonstrate the possibility of the formation of a vortex state in YBCO and its evolution with increasing BB.
The effect of high-energy electron irradiation on the temperature dependences of the resistivity ρ(T)\rho(T), fluctuation conductivity (FLC), and pseudogap (PG) Δ(T)\Delta^{*}(T) of YBa2_2Cu3_3O7_7--δ\delta (YBCO) single crystals without twins was studied. Irradiation causes a linear increase in ρ(T)\rho(T) and a decrease in the superconducting transition temperature TcT_c with dose ϕ\phi. For small ϕ\phi, the reduction of TcT_c follows the Abrikosov--Gorkov (AG) pair-breaking theory, while for large ϕ\phi it is described by the Emery--Kivelson (EK) model, where quantum phase fluctuations dominate. At ϕ3=2.5×1019\phi_3 = 2.5 \times 10^{19} e/cm2^2, which corresponds to the AG--EK crossover, the spacing between CuO2_2 planes d01d_{01}, the coherence length ξc(0)\xi_c(0), and the fluctuation region TflT_{\mathrm{fl}} increase sharply, and the two-dimensional Maki--Thompson (2D--MT) contribution is replaced by the Aslamazov--Larkin (2D--AL) term. Surprisingly, no signatures of the crossover appear in ρ(ϕ)\rho(\phi) or Tc(ϕ)T_c(\phi). At the same ϕ3\phi_3, a sharp rise in the pseudogap opening temperature TT^{*} and in Δ\Delta^{*} indicates a possible reduction of the density of states. With further increase in ϕ\phi, both PG parameters and their energy scale decrease markedly, and Δ(T)\Delta^{*}(T) acquires an unusual form. However, at ϕ5=5.6×1019\phi_5 = 5.6 \times 10^{19} e/cm2^2, the temperature dependences of FLC and PG again show behavior typical of well-structured YBCO, regardless of defect density.
The temperature dependences of both fluctuation conductivity (FLC) σ(T)\sigma^\prime(T) and pseudogap (PG) Δ(T)\Delta^*(T) derived from measurements of resistivity ρ(T)\rho(T) of an optimally doped YBa2_2Cu3_3O7δ_{7-\delta} single crystal subjected to long-term storage have been studied. The as-grown sample S1 exhibits characteristics typical of optimally doped YBa2_2Cu3_3O7δ_{7-\delta} single crystals containing twins and twin boundaries. Analysis of both FLC and PG showed an unexpected improvement in all characteristics of the sample after 6 years of storage (sample S2), indicating that the effect of twin boundaries is somehow limited. After 17 years of storage, all characteristics of the sample changed dramatically, which indicates a strong influence of internal defects formed during the aging process. For the first time, the temperature dependences of both FLC and PG were obtained after 17 years of storage.
We study the interplay between superconductivity and altermagnetism in disordered systems using recently derived quantum kinetic transport equations. Starting from this framework, we derive the Ginzburg-Landau free energy and identify, in addition to the conventional pair-breaking term, a coupling between the spin and the spatial variation of the superconducting order parameter. Two distinct effects emerge from this coupling. The first is a magnetoelectric effect, in which a supercurrent (i.e., a phase gradient) induces a spin texture; this contribution is quadratic in the phase gradient. The second effect arises when the magnitude, rather than the phase, of the superconducting order parameter varies in space, likewise leading to a finite magnetization. We show that these two contributions compete in the case of an Abrikosov vortex, where both the amplitude and phase of the order parameter vary spatially. The effect associated with amplitude variations also gives rise to a proximity-induced magnetization (PIM) in hybrid structures composed of a superconductor (S) and an altermagnet (AM). Using quasiclassical theory, we analyze the PIM in diffusive S/AM bilayers and S/AM/S Josephson junctions, and determine the induced magnetization profiles. In Josephson junctions, where both the PIM and the magnetoelectric effect coexist, we further predict the occurrence of 00-π\pi transitions.
Freestanding thin films, a class of low-dimensional materials capable of maintaining structural integrity without substrates, have emerged as a forefront research focus. Their unique advantages-circumventing substrate clamping, liberating intrinsic material properties, and enabling cross-platform heterogeneous integration-underpin this prominence. This review systematically summarizes core fabrication techniques, including physical delamination (e.g., laser lift-off, mechanical exfoliation) and chemical etching, alongside associated transfer strategies. It further explores the induced strain modulation mechanisms, extreme mechanical properties and interface decoupling effects enabled by these films. Representative case studies demonstrate breakthrough applications in flexible/ultrathin electronics, ultrahigh-sensitivity sensors and the exploration of novel quantum states. Critical challenges regarding scalable fabrication, precise interface control, and long-term stability are analyzed, concluding with prospects for emerging applications in bio-inspired intelligent devices, quantum precision sensing, and brain-inspired neural networks.
Recent observations of superconductivity in twisted bilayer WSe2_2 have extended the family of moiré superconductors beyond twisted graphene. In WSe2_2 two different twist angles were studied, 3.65° and 5.0°, and two seemingly distinct superconducting phase diagrams were reported, raising the question of whether the superconducting phases in the two devices share a similar origin. Here we address the question by experimentally mapping the evolution of the phase diagram across devices with twist angles spanning the range defined by the initial reports, and comparing the results to twist angle-dependent theory. We find that the superconducting state evolves smoothly with twist angle and at all twist angles is proximal to a Fermi surface reconstruction with, presumably, antiferromagnetic ordering, but is neither necessarily tied to the Van Hove singularity, nor to the half band insulator. Our results connect the previously distinct phase diagrams at 3.65° and 5°, and offer new insight into the origin of the superconductivity in this system and its evolution as the correlation strength increases. More broadly, the smooth phase diagram evolution, repeatability between different devices, and dynamic gate tunability within each device, establish twisted transition metal dichalcogenides as a unique platform for the study of correlated phases as the ratio of interaction strength to bandwidth is varied.
There are multiple possible origins of transport anisotropies in metals and superconductors. For instance, rotational symmetry can be spontaneously broken in the normal state as a result of electronic nematic order inducing anisotropies in an otherwise ss-wave superconducting phase. Another possibility is that the dominant source of rotational symmetry breaking is the superconductor itself and its vestiges that may survive in the normal state. We here theoretically analyze the correlations of transport anisotropies in the normal and the corresponding superconducting phase for different scenarios of broken symmetry, either coming solely from the normal state, solely from the superconductor and its vestiges in the metallic regimes, or from both simultaneously. We further include both zero-momentum and finite-momentum pairing; we develop a theory of vestigial order for the latter, characterized by broken rotational and translational symmetry. Our findings reveal that the relative transport anisotropies in the normal and superconducting phases sensitively depend on the scenario, including the form of vestigial order and, in some cases, the parity of the superconducting order parameter. As such, measuring the directional dependence of the critical current and resistivity can provide strong constraints on the origin of rotational symmetry breaking. We demonstrate our findings in minimal models relevant to twisted multilayer graphene, rhombohedral graphene, and twisted transition metal dichalcogenides.
Cr1/3_{1/3}NbS2_{2} is a transition metal dichalcogenide that is also a chiral helimagnet, and so lacks inversion symmetry and has non-zero Berry curvature in position and momentum space. It is well known that the combination of broken time-reversal symmetry and broken inversion symmetry can generate non-reciprocal phenomena, but the interplay between these kinds of systems and superconductivity is not well known. We present Josephson junctions fabricated from Cr1/3_{1/3}NbS2_{2} that give magnetic diffraction patterns with asymmetry in both the magnetic field and the critical current. The non-reciprocity in positive critical current and negative critical current, generally called the Josephson diode effect, has an efficiency of up to η=20%\eta=20\% in some parts of the magnetic diffraction pattern and persists even at zero applied field. We propose that pinned Abrikosov vortices are a main mechanism for the asymmetric magnetic field response in this system, and that the non-zero spin chirality of the Cr1/3_{1/3}NbS2_{2} causes the diode effect. Simulations of magnetic diffraction patterns from Josephson junctions with vortices present show offsets from zero-field consistent with observations, while simulations of chiral spin structures with an out-of-plane canting show a diode effect.
We report the first experimental realization of a scalable basic cell for quantum routing, enabling coherent control and exchange of microwave photons between two spatially separated superconducting waveguides coupled via a single transmon qubit. The cell was characterized at 10 mK with an average input signal of approximately 1 photon at approximately 6 GHz, and with the qubit biased to its optimal point to minimize sensitivity to external magnetic fluctuations. By combining steady-state and time-domain measurements, we reconstructed the key parameters of the system, including qubit relaxation and dephasing, waveguide-qubit couplings, and cross-waveguide photon transfer efficiency. The observed performance is consistent with a non-Hermitian Hamiltonian formalism and demonstrates clear limits set by flux bias, temperature, and photon number, in agreement with flux- and temperature-induced dephasing models. Crucially, the cell operates reliably at the single-photon level, and in the high-photon regime we directly observe photon dressing induced by the qubit. These results establish a versatile platform for studying open quantum system phenomena and pave the way for scalable implementations of quantum routing and network nodes.
The two-dimensional (2D) Hubbard model has long attracted interest for its rich phase diagram and its relevance to high-TcT_c superconductivity. However, reliable finite-temperature studies remain challenging due to the exponential complexity of many-body interactions. Here, we introduce an enhanced 1s+1\text{s}^+ eXponential Tensor Renormalization Group algorithm that enables efficient finite-temperature simulations of the 2D Hubbard model. By exploring an expanded space, our approach achieves two-site update accuracy at the computational cost of a one-site update, and delivers up to 50% acceleration for Hubbard-like systems, which enables simulations down to T ⁣ ⁣0.004tT\!\approx\!0.004t. This advance permits a direct investigation of superconducting order over a wide temperature range and facilitates a comparison with zero-temperature infinite Projected Entangled Pair State simulations. Finally, we compile a comprehensive dataset of snapshots spanning the relevant region of the phase diagram, providing a valuable reference for Artificial Intelligence-driven analyses of the Hubbard model and a comparison with cold-atom experiments.
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