The one-dimensional Fr\"ohlich model describing the motion of a single electron interacting with optical phonons is a paradigmatic model of quantum many-body physics. We predict the existence of an arbitrarily large number of bound excited states in the strong coupling limit and calculate their excitation energies. Numerical simulations of a discretized model demonstrate the complete amelioration of the projector Monte Carlo sign problem by walker annihilation in an infinite Hilbert space. They reveal the threshold for the occurrence of the first bound excited states at a value of $\alpha \approx 1.73$ for the dimensionless coupling constant. This puts the threshold into the regime of intermediate interaction strength. We calculate the spectral weight and the number density of the dressing cloud in the discretized model.

Recently, it was shown that quantum interference in a system containing a polarized and unpolarized emitter can allow directional emission of photons into a circulating cavity. Here, we ask whether high directionality of photon emission in this system implies a high degree of quantum correlation between the two emitters. We show that the answer is a qualified "yes", with photon emission directionality and emitter-emitter entanglement showing a monotonic relationship over a broad parameter range. The relationship only breaks down in the limit of perfect directionality. Furthermore, under reasonable assumptions for experimental parameters and stability, we show that the statistics of measured directionality allow a reliable estimate of the concurrence. This result implies that directionality of photon emission in the state preparation stage can be used to determine the entanglement between the emitters, with potential applications to more generic cases including quantum networks.

We report on the synthesis and spectroscopic characterization of Sm$^{3+}$-doped K$_2$YF$_5$ microparticles. The particles were synthesized via the hydrothermal technique, yielding a particle size of approximately 20 $\mu$m in length. Scanning electron microscopy (SEM) and X-ray diffraction (XRD) analyses confirmed their orthorhombic crystal structure. A combination of absorption and laser excited fluorescence performed on samples cooled to 10~K, allow for the determination of {56} experimental crystal-field levels. A parametrised crystal-field analysis for Sm$^{3+}$ in the C$_{\rm s}$ point group symmetry centres of K$_2$YF$_5$ yields good approximation to the data.

Recent experiments with degenerate molecular gases dressed by elliptically polarized microwave fields have opened new avenues for engineering dipolar interactions. We identify a set of symmetries of the interaction potential, which generate degeneracies among the interaction parameters, and use these to classify the resulting spatial symmetries and equilibrium shapes of the gases. Exploiting these symmetries we analyze solutions including beyond-meanfield quantum fluctuations, and develop complementary variational results. We then map out the phase diagram of self-bound droplets and characterize their key properties.

We demonstrate protected single-soliton formation and operation in a Kerr microresonator using a phase-modulated pump laser. Phase modulation gives rise to spatially varying effective loss and detuning parameters, which in turn lead to an operation regime in which multi-soliton degeneracy is lifted and a single soliton is the only observable behavior. Direct excitation of single solitons is indicated by observed reversal of the characteristic 'soliton step.' Phase modulation also enables precise control of the soliton pulse train's properties, and measured dynamics agree closely with simulations. We show that the technique can be extended to high repetition-frequency Kerr solitons through subharmonic phase modulation. These results facilitate straightforward generation and control of Kerr-soliton microcombs for integrated photonics systems.

We demonstrate protected single-soliton formation and operation in a Kerr microresonator using a phase-modulated pump laser. Phase modulation gives rise to spatially varying effective loss and detuning parameters, which in turn lead to an operation regime in which multi-soliton degeneracy is lifted and a single soliton is the only observable behavior. Direct excitation of single solitons is indicated by observed reversal of the characteristic 'soliton step.' Phase modulation also enables precise control of the soliton pulse train's properties, and measured dynamics agree closely with simulations. We show that the technique can be extended to high repetition-frequency Kerr solitons through subharmonic phase modulation. These results facilitate straightforward generation and control of Kerr-soliton microcombs for integrated photonics systems.

This is the second article in a series of two which report on a matrix approach for ultrasound imaging in heterogeneous media. This article describes the quantification and correction of aberration, i.e. the distortion of an image caused by spatial variations in the medium speed-of-sound. Adaptive focusing can compensate for aberration, but is only effective over a restricted area called the isoplanatic patch. Here, we use an experimentally-recorded matrix of reflected acoustic signals tosynthesize a set of virtual transducers. We then examine wave propagation between these virtual transducers and an arbitrary correction plane. Such wave-fronts consist of two components: (i) An ideal geometric wave-front linked to diffraction and the input focusing point, and; (ii) Phase distortions induced by the speed-of-sound variations. These distortions are stored in a so-called distortion matrix, the singular value decomposition of which gives access to an optimized focusing law at any point. We show that, by decoupling the aberrations undergone by the outgoing and incoming waves and applying an iterative strategy, compensation for even high-order and spatially-distributed aberrations can be achieved. After a numerical validation of the process, ultrasound matrix imaging (UMI) is applied to the in-vivo imaging of a gallbladder. A map of isoplanatic modes is retrieved and is shown to be strongly correlated with the arrangement of tissues constituting the medium. The corresponding focusing laws yield an ultrasound image with drastically improved contrast and transverse resolution. UMI thus provides a flexible and powerful route towards computational ultrasound.

This is the second article in a series of two which report on a matrix approach for ultrasound imaging in heterogeneous media. This article describes the quantification and correction of aberration, i.e. the distortion of an image caused by spatial variations in the medium speed-of-sound. Adaptive focusing can compensate for aberration, but is only effective over a restricted area called the isoplanatic patch. Here, we use an experimentally-recorded matrix of reflected acoustic signals tosynthesize a set of virtual transducers. We then examine wave propagation between these virtual transducers and an arbitrary correction plane. Such wave-fronts consist of two components: (i) An ideal geometric wave-front linked to diffraction and the input focusing point, and; (ii) Phase distortions induced by the speed-of-sound variations. These distortions are stored in a so-called distortion matrix, the singular value decomposition of which gives access to an optimized focusing law at any point. We show that, by decoupling the aberrations undergone by the outgoing and incoming waves and applying an iterative strategy, compensation for even high-order and spatially-distributed aberrations can be achieved. After a numerical validation of the process, ultrasound matrix imaging (UMI) is applied to the in-vivo imaging of a gallbladder. A map of isoplanatic modes is retrieved and is shown to be strongly correlated with the arrangement of tissues constituting the medium. The corresponding focusing laws yield an ultrasound image with drastically improved contrast and transverse resolution. UMI thus provides a flexible and powerful route towards computational ultrasound.

We simulate the Gross-Pitaevskii equation to model the development of turbulence in a quantum fluid confined by a cuboid box potential, and forced by shaking along one axis. We observe the development of isotropic turbulence from anisotropic forcing for a broad range of forcing amplitudes, and characterise the states through their Fourier spectra, vortex distributions, and spatial correlations. For weak forcing the steady-state wave-action spectrum exhibits a $k^{-3.5}$ scaling over wavenumber $k$; further decomposition uncovers the same power law in both compressible kinetic energy and quantum pressure, while the bulk superfluid remains phase coherent and free from extended vortices. As the forcing energy exceeds the chemical potential, extended vortices develop in the bulk, disrupting the $k^{-3.5}$ scaling. The spectrum then transitions to a $k^{-7/3}$ regime for compressible kinetic energy only, associated with dense vortex turbulence, and phase coherence limited to the healing length. The strong forcing regime is consistent with an inverse cascade of compressible energy driven by small-scale vortex annihilation.

This is the first article in a series of two dealing with a matrix approach for aberration quantification and correction in ultrasound imaging. Advanced synthetic beamforming relies on a double focusing operation at transmission and reception on each point of the medium. Ultrasound matrix imaging (UMI) consists in decoupling the location of these transmitted and received focal spots. The response between those virtual transducers form the so-called focused reflection matrix that actually contains much more information than a confocal ultrasound image. In this paper, a time-frequency analysis of this matrix is performed, which highlights the single and multiple scattering contributions as well as the impact of aberrations in the monochromatic and broadband regimes. Interestingly, this analysis enables the measurement of the incoherent input-output point spread function at any pixel of this image. A fitting process enables the quantification of the single scattering, multiple scattering and noise components in the image. From the single scattering contribution, a focusing criterion is defined, and its evolution used to quantify the amount of aberration throughout the ultrasound image. In contrast to the state-of-the-art coherence factor, this new indicator is robust to multiple scattering and electronic noise, thereby providing a contrasted map of the focusing quality at a much better transverse resolution. After a validation of the proof-of-concept based on time-domain simulations, UMI is applied to the in-vivo study of a human calf. Beyond this specific example, UMI opens a new route for speed-of-sound and scattering quantification in ultrasound imaging.

Quantum entanglement is usually considered a fragile quantity and decoherence through coupling to an external environment, such as a thermal reservoir, can quickly destroy the entanglement resource. This doesn't have to be the case and the environment can be engineered to assist in the formation of entanglement. We investigate a system of qubits and higher dimensional spins interacting only through their mutual coupling to a reservoir. We explore the entanglement of multipartite and multidimensional system as mediated by the bath and show that at low temperatures and intermediate coupling strengths multipartite entanglement may form between qubits and between higher spins, i.e., qudits. We characterise the multipartite entanglement using an entanglement witness based upon the structure factor and demonstrate its validity versus the directly calculated entanglement of formation, suggesting possible experiments for its measure.

This is the first article in a series of two dealing with a matrix approach for aberration quantification and correction in ultrasound imaging. Advanced synthetic beamforming relies on a double focusing operation at transmission and reception on each point of the medium. Ultrasound matrix imaging (UMI) consists in decoupling the location of these transmitted and received focal spots. The response between those virtual transducers form the so-called focused reflection matrix that actually contains much more information than a confocal ultrasound image. In this paper, a time-frequency analysis of this matrix is performed, which highlights the single and multiple scattering contributions as well as the impact of aberrations in the monochromatic and broadband regimes. Interestingly, this analysis enables the measurement of the incoherent input-output point spread function at any pixel of this image. A fitting process enables the quantification of the single scattering, multiple scattering and noise components in the image. From the single scattering contribution, a focusing criterion is defined, and its evolution used to quantify the amount of aberration throughout the ultrasound image. In contrast to the state-of-the-art coherence factor, this new indicator is robust to multiple scattering and electronic noise, thereby providing a contrasted map of the focusing quality at a much better transverse resolution. After a validation of the proof-of-concept based on time-domain simulations, UMI is applied to the in-vivo study of a human calf. Beyond this specific example, UMI opens a new route for speed-of-sound and scattering quantification in ultrasound imaging.

We report on the synthesis and spectroscopic characterization of Sm$^{3+}$-doped K$_2$YF$_5$ microparticles. The particles were synthesized via the hydrothermal technique, yielding a particle size of approximately 20 $\mu$m in length. Scanning electron microscopy (SEM) and X-ray diffraction (XRD) analyses confirmed their orthorhombic crystal structure. A combination of absorption and laser excited fluorescence performed on samples cooled to 10~K, allow for the determination of {56} experimental crystal-field levels. A parametrised crystal-field analysis for Sm$^{3+}$ in the C$_{\rm s}$ point group symmetry centres of K$_2$YF$_5$ yields good approximation to the data.

We focus on the existence and persistence of families of saddle periodic orbits in a four-dimensional Hamiltonian reversible ordinary differential equation derived using a travelling wave ansatz from a generalised nonlinear Schr{ö}dinger equation (GNLSE) with quartic dispersion. In this way, we are able to characterise different saddle periodic orbits with different signatures that serve as organising centres of homoclinic orbits in the ODE and solitons in the GNLSE. To achieve our objectives, we employ numerical continuation techniques to compute these saddle periodic orbits, and study how they organise themselves as surfaces in phase space that undergo changes as a single parameter is varied. Notably, different surfaces of saddle periodic orbits can interact with each other through bifurcations that can drastically change their overall geometry or even create new surfaces of periodic orbits. Particularly we identify three different bifurcations: symmetry-breaking, period-$k$ multiplying, and saddle-node bifurcations. Each bifurcation exhibits a degenerate case, which subsequently gives rise to two bifurcations of the same type that occurs at particular energy levels that vary as a parameter is gradually increased. Additionally, we demonstrate how these degenerate bifurcations induce structural changes in the periodic orbits that can support homoclinic orbits by computing sequences of period-$k$ multiplying bifurcations.

We develop a theoretical description of a device for coherent conversion of microwave to optical photons. For the device, dopant ions in a crystal are used as three-level systems, and interact with the fields inside overlapping microwave and optical cavities. We develop a model for the cavity fields interacting with an ensemble of ions, and model the ions using an open quantum systems approach, while accounting for the effect of inhomogeneous broadening. Numerical methods are developed to allow us to accurately simulate the device. We also further develop a simplified model, applicable in the case of small cavity fields which is relevant to quantum information applications. This simplified model is used to predict the maximum conversion efficiency of the device. We investigate the effect of various parameters, and predict that conversion efficiency of above 80% should be possible with currently existing experimental setups inside a dilution refrigerator.

We predict a rich excitation spectrum of a binary dipolar supersolid in a linear crystal geometry, where the ground state consists of two partially immiscible components with alternating, interlocking domains. We identify three Goldstone branches, each with first-sound, second-sound or spin-sound character. In analogy with a diatomic crystal, the resulting lattice has a two-domain primitive basis and we find that the crystal (first-sound-like) branch is split into optical and acoustic phonons. We also find a spin-Higgs branch that is associated with the supersolid modulation amplitude.

In recent years there have been significant advances in the study of many-body interactions between atoms and light confined to optical cavities. One model which has received widespread attention of late is the Dicke model, which under certain conditions exhibits a quantum phase transition to a state in which the atoms collectively emit light into the cavity mode, known as superradiance. We consider a generalization of this model that features independently controllable strengths of the co- and counter-rotating terms of the interaction Hamiltonian. We study this system in the semiclassical (mean field) limit, i.e., neglecting the role of quantum fluctuations. Under this approximation, the model is described by a set of nonlinear differential equations, which determine the system's semiclassical evolution. By taking a dynamical systems approach, we perform a comprehensive analysis of these equations to reveal an abundance of novel and complex dynamics. Examples of the novel phenomena that we observe are the emergence of superradiant oscillations arising due to Hopf bifurcations, and the appearance of a pair of chaotic attractors arising from period-doubling cascades, followed by their collision to form a single, larger chaotic attractor via a sequence of infinitely many homoclinic bifurcations. Moreover, we find that a flip of the collective spin can result in the sudden emergence of chaotic dynamics. Overall, we provide a comprehensive roadmap of the possible dynamics that arise in the unbalanced, open Dicke model in the form of a phase diagram in the plane of the two interaction strengths. Hence, we lay out the foundations to make further advances in the study of the fingerprint of semiclassical chaos when considering the master equation of the unbalanced Dicke model, that is, the possibility of studying a manifestation of quantum chaos in a specific, experimentally realizable system.

Rydberg atoms efficiently link photons between the radio-frequency (RF) and optical domains. They furnish a medium in which the presence of an RF field imprints on the transmission of a probe laser beam by altering the coherent coupling between atomic quantum states. The immutable atomic energy structure underpins quantum-metrological RF field measurements and has driven intensive efforts to realize inherently self-calibrated sensing devices. Here we investigate spectroscopic signatures owing to the angular momentum quantization of the atomic states utilized in an electromagnetically-induced transparency (EIT) sensing scheme for linearly polarized RF fields. Specific combinations of atomic terms are shown to give rise to universal, distinctive fingerprints in the detected optical fields upon rotating the RF field polarization. Using a dressed state picture, we identify two types of atomic angular momentum ladders that display strikingly disparate spectroscopic signatures, including the complementary absence or presence of a central spectral EIT peak. Our study adds important insights into the prospects of Rydberg atomic gases for quantum metrological electric field characterization. In particular, it calls into question prevailing interpretations of SI-traceable Rydberg atom electrometers.

We investigate the Autler-Townes splitting for Rydberg atoms dressed with linearly polarized microwave radiation, resonant with generic $S_{1/2}\leftrightarrow{P}_{1/2}$ and $S_{1/2}\leftrightarrow{P}_{3/2}$ transitions. The splitting is probed using laser light via electromagnetically-induced transparency measurements, where the transmission of probe laser light reveals a two-peak pattern. In particular, this pattern is invariant under rotation of the microwave field polarization. In consequence, we establish $S \leftrightarrow P$ Rydberg transitions as ideally suited for polarization-insensitive electrometry, contrary to recent findings [A. Chopinaud and J.D. Pritchard, Phys. Rev. Appl. $\mathbf{16}$, 024008 (2021)].

We develop a new theoretical framework for exploring a mobile impurity interacting strongly with a highly correlated bath of bosons in the quantum critical regime of a Mott insulator (MI) to superfluid (SF) quantum phase transition. Our framework is based on a powerful quantum Gutzwiller (QGW) description of the bosonic bath combined with diagrammatic field theory for the impurity-bath interactions. By resumming a selected class of diagrams to infinite order, a rich picture emerges where the impurity is dressed by the fundamental modes of the bath, which change character from gapped particle-hole excitations in the MI to Higgs and gapless Goldstone modes in the SF. This gives rise to the existence of several quasiparticle (polaron) branches with properties reflecting the strongly correlated environment. In particular, one polaron branch exhibits a sharp cusp in its energy, while a new ground-state polaron emerges at the $O(2)$ quantum phase transition point for integer filling, which reflects the nonanalytic behavior at the transition and the appearance of the Goldstone mode in the SF phase. Smooth versions of these features are inherited in the polaron spectrum away from integer filling because of the varying ``Mottness" of the bosonic bath. We furthermore compare our diagrammatic results with quantum Monte Carlo calculations, obtaining excellent agreement. This accuracy is quite remarkable for such a highly non-trivial case of strong interactions between the impurity and bosons in a maximally correlated quantum critical regime, and it establishes the utility of our framework. Finally, our results show how impurities can be used as quantum sensors and highlight fundamental differences between experiments performed at a fixed particle number or a fixed chemical potential.