ICREA - Instituci ́o Catalana de Recerca i Estudis Avan ̧cats
Spin Hall effects are a collection of relativistic spin-orbit coupling phenomena in which electrical currents can generate transverse spin currents and vice versa. Although first observed only a decade ago, these effects are already ubiquitous within spintronics as standard spin-current generators and detectors. Here we review the experimental and theoretical results that have established this sub-field of spintronics. We focus on the results that have converged to give us a clear understanding of the phenomena and how they have evolved from a qualitative to a more quantitative measurement of spin-currents and their associated spin-accumulation. Within the experimental framework, we review optical, transport, and magnetization-dynamics based measurements and link them to both phenomenological and microscopic theories of the effect. Within the theoretical framework, we review the basic mechanisms in both the extrinsic and intrinsic regime which are linked to the mechanisms present in their closely related phenomenon in ferromagnets, the anomalous Hall effect. We also review the connection to the phenomenological treatment based on spin-diffusion equations applicable to certain regimes, as well as the spin-pumping theory of spin-generation which has proven important in the measurements of the spin Hall angle. We further connect the spin-current generating spin Hall effect to the inverse spin galvanic effect, which often accompanies the SHE, in which an electrical current induces a non-equilibrium spin polarization. These effects share common microscopic origins and can exhibit similar symmetries when present in ferromagnetic/non-magnetic structures through their induced current-driven spin torques. Although we give a short chronological overview, the main body is structured from a pedagogical point of view, focusing on well-established and accepted physics.
Tremendous progress in experimental quantum optics during the past decades enabled the advent of quantum technologies, one of which is quantum communication. Aimed at novel methods for more secure or efficient information transfer, quantum communication has developed into an active field of research and proceeds toward full-scale implementations and industrialization. Continuous-variable methods of multi-photon quantum state preparation, manipulation, and coherent detection, as well as the respective theoretical tools of phase-space quantum optics, offer the possibility to make quantum communication efficient, applicable and accessible, thus boosting the development of the field. We review the methodology, techniques and protocols of continuous-variable quantum communication, from the first theoretical ideas, through milestone implementations, to the recent developments, covering quantum key distribution as well as other quantum communication schemes, suggested on the basis of continuous-variable states and measurements.
A fundamental problem in quantum thermodynamics is to properly quantify the work extractable from out-of-equilibrium systems. While for closed systems, maximum quantum work extraction is defined in terms of the ergotropy functional, this question is unclear in open systems interacting with an environment. The concept of local ergotropy has been proposed, but it presents several problems, such as it is not guaranteed to be non-increasing in time. Here we introduce the concept of extended local ergotropy by exploiting the free evolution of the system-environment compound. At variance with the local ergotropy, the extended local ergotropy is greater, is non-increasing in time, and activates the potential of work extraction in many cases. We then concentrate on specific schemes in which we alternate repeated local unitaries and free system-environment evolution. We provide examples based on the Jaynes-Cummings model, presenting practical protocols and analytic results that serve as proof of principle for the aforementioned advantages.
In this paper we study the subset of generalized quantum measurements on finite dimensional systems known as local operations and classical communication (LOCC). While LOCC emerges as the natural class of operations in many important quantum information tasks, its mathematical structure is complex and difficult to characterize. Here we provide a precise description of LOCC and related operational classes in terms of quantum instruments. Our formalism captures both finite round protocols as well as those that utilize an unbounded number of communication rounds. While the set of LOCC is not topologically closed, we show that finite round LOCC constitutes a compact subset of quantum operations. Additionally we show the existence of an open ball around the completely depolarizing map that consists entirely of LOCC implementable maps. Finally, we demonstrate a two-qubit map whose action can be approached arbitrarily close using LOCC, but nevertheless cannot be implemented perfectly.
In this paper we analyze a suite of cosmological simulations of modified gravitational action f(R) models, where cosmic acceleration is induced by a scalar field that acts as a fifth force on all forms of matter. In particular, we focus on the bispectrum of the dark matter density field on mildly non-linear scales. For models with the same initial power spectrum, the dark matter bispectrum shows significant differences for cases where the final dark matter power spectrum also differs. Given the different dependence on bias of the galaxy power spectrum and bispectrum, bispectrum measurements can close the loophole of galaxy bias hiding differences in the power spectrum. Alternatively, changes in the initial power spectrum can also hide differences. By constructing LCDM models with very similar final non-linear power spectra, we show that the differences in the bispectrum are reduced (<4%) and are comparable with differences in the imperfectly matched power spectra. These results indicate that the bispectrum depends mainly on the power spectrum and less sensitively on the gravitational signatures of the f(R) model. This weak dependence of the matter bispectrum on gravity makes it useful for breaking degeneracies associated with galaxy bias, even for models beyond general relativity.
Among several tasks in Machine Learning, a specially important one is that of inferring the latent variables of a system and their causal relations with the observed behavior. Learning a Hidden Markov Model of given stochastic process is a textbook example, known as the positive realization problem (PRP). The PRP and its solutions have far-reaching consequences in many areas of systems and control theory, and positive systems theory. We consider the scenario where the latent variables are quantum states, and the system dynamics is constrained only by physical transformations on the quantum system. The observable dynamics is then described by a quantum instrument, and the task is to determine which quantum instrument --if any-- yields the process at hand by iterative application. We take as starting point the theory of quasi-realizations, whence a description of the dynamics of the process is given in terms of linear maps on state vectors and probabilities are given by linear functionals on the state vectors. This description, despite its remarkable resemblance with the Hidden Markov Model, or the iterated quantum instrument, is nevertheless devoid of any stochastic or quantum mechanical interpretation, as said maps fail to satisfy any positivity conditions. The Completely-Positive realization problem then consists in determining whether an equivalent quantum mechanical description of the same process exists. We generalize some key results of stochastic realization theory, and show that the problem has deep connections with operator systems theory, yielding possible insight to the lifting problem in quotient operator systems. Our results have potential applications in quantum machine learning, device-independent characterization and reverse-engineering of stochastic processes and quantum processors, and dynamical processes with quantum memory.
We use a recently discovered constrained de Finetti reduction (aka "Post-Selection Lemma") to study the parallel repetition of multi-player non-local games under no-signalling strategies. Since the technique allows us to reduce general strategies to independent plays, we obtain parallel repetition (corresponding to winning all rounds) in the same way as exponential concentration of the probability to win a fraction larger than the value of the game. Our proof technique leads us naturally to a relaxation of no-signalling (NS) strategies, which we dub sub-no-signalling (SNOS). While for two players the two concepts coincide, they differ for three or more players. Our results are most complete and satisfying for arbitrary number of sub-no-signalling players, where we get universal parallel repetition and concentration for any game, while the no-signalling case is obtained as a corollary, but only for games with "full support".
We present a non-perturbative numerical technique for calculating strong light shifts in atoms under the influence of multiple optical fields with arbitrary polarization. We confirm our technique experimentally by performing spectroscopy of a cloud of cold 87^{87}Rb atoms subjected to \sim kW/cm2^2 intensities of light at 1560.492 nm simultaneous with 1529.269 nm or 1529.282 nm. In these conditions the excited state resonances at 1529.26 nm and 1529.36 nm induce strong level mixing and the shifts are highly nonlinear. By absorption spectroscopy, we observe that the induced shifts of the 5P3/2 hyperfine Zeeman sublevels agree well with our theoretical predictions.. We propose the application of our theory and experiment to accurate measurements of excited-state electric-dipole matrix elements.
We investigate the fundamental limitations imposed by thermodynamics for creating correlations. Considering a collection of initially uncorrelated thermal quantum systems, we ask how much classical and quantum correlations can be obtained via a cyclic Hamiltonian process. We derive bounds on both the mutual information and entanglement of formation, as a function of the temperature of the systems and the available energy. While for a finite number of systems there is a maximal temperature allowing for the creation of entanglement, we show that genuine multipartite entanglement---the strongest form of entanglement in multipartite systems---can be created at any temperature when sufficiently many systems are considered. This approach may find applications, e.g. in quantum information processing, for physical platforms in which thermodynamic considerations cannot be ignored.
The driven Dicke model, wherein an ensemble of atoms is driven by an external field and undergoes collective spontaneous emission due to coupling to a leaky cavity mode, is a paradigmatic example of a system exhibiting a driven-dissipative phase transition as a function of driving strength. Recently, a similar phenomenon was experimentally observed, not in a cavity setting, but rather in a free-space atomic ensemble. The reason why similar behavior should emerge in free space is not obvious, as the system interacts with a continuum of optical modes, which encodes light propagation effects. Here, we present and solve a simple model to explain the behavior of the free-space system, based on the one-dimensional Maxwell-Bloch equations. On one hand, we show that a free-space ensemble at a low optical depth can exhibit similar behavior as the cavity system, as spatial propagation effects are negligible. On the other hand, in the thermodynamic limit of large atom number, we show that certain observables such as the transmittance or the atomic excited population exhibit non-analytic behavior as a function of the driving intensity, reminiscent of a phase transition. However, a closer analysis reveals that the atomic properties are highly inhomogeneous in space, and based on this we argue that the free-space system does not undergo a phase transition but rather a ``phase separation", roughly speaking, between saturated and unsaturated regions.
We show that a relatively simple reasoning using von Neumann entropy inequalities yields a robust proof of the quantum Singleton bound for quantum error-correcting codes (QECC). For entanglement-assisted quantum error-correcting codes (EAQECC) and catalytic codes (CQECC), a type of generalized quantum Singleton bound [Brun et al., IEEE Trans. Inf. Theory 60(6):3073--3089 (2014)] was believed to hold for many years until recently one of us found a counterexample [MG, Phys. Rev. A 103, 020601 (2021)]. Here, we rectify this state of affairs by proving the correct generalized quantum Singleton bound, extending the above-mentioned proof method for QECC; we also prove information-theoretically tight bounds on the entanglement-communication tradeoff for EAQECC. All of the bounds relate block length nn and code length kk for given minimum distance dd and we show that they are robust, in the sense that they hold with small perturbations for codes which only correct most of the erasure errors of less than dd letters. In contrast to the classical case, the bounds take on qualitatively different forms depending on whether the minimum distance is smaller or larger than half the block length. We also provide a propagation rule: any pure QECC yields an EAQECC with the same distance and dimension, but of shorter block length.
An optical quantum memory can be broadly defined as a system capable of storing a useful quantum state through interaction with light at optical frequencies. During the last decade, intense research was devoted to their development, mostly with the aim of fulfilling the requirements of their first two applications, namely quantum repeaters and linear-optical quantum computation. A better understanding of those requirements then motivated several different experimental approaches. Along the way, other exciting applications emerged, such as as quantum metrology, single-photon detection, tests of the foundations of quantum physics, device-independent quantum information processing and nonlinear processing of quantum information. Here we review several prospective applications of optical quantum memories with a focus on recent experimental achievements pertaining to these applications. This review highlights that optical quantum memories have become essential for the development of optical quantum information processing.
The unpredictability of random numbers is fundamental to both digital security and applications that fairly distribute resources. However, existing random number generators have limitations-the generation processes cannot be fully traced, audited, and certified to be unpredictable. The algorithmic steps used in pseudorandom number generators are auditable, but they cannot guarantee that their outputs were a priori unpredictable given knowledge of the initial seed. Device-independent quantum random number generators can ensure that the source of randomness was unknown beforehand, but the steps used to extract the randomness are vulnerable to tampering. Here, for the first time, we demonstrate a fully traceable random number generation protocol based on device-independent techniques. Our protocol extracts randomness from unpredictable non-local quantum correlations, and uses distributed intertwined hash chains to cryptographically trace and verify the extraction process. This protocol is at the heart of a public traceable and certifiable quantum randomness beacon that we have launched. Over the first 40 days of operation, we completed the protocol 7434 out of 7454 attempts -- a success rate of 99.7%. Each time the protocol succeeded, the beacon emitted a pulse of 512 bits of traceable randomness. The bits are certified to be uniform with error times actual success probability bounded by 2642^{-64}. The generation of certifiable and traceable randomness represents one of the first public services that operates with an entanglement-derived advantage over comparable classical approaches.
Noncollinear magnets are notoriously difficult to describe within first-principles approaches based on density-functional theory (DFT) because of the presence of low-lying spin excitations. At the level of ground-state calculations, several methods exist to constrain the magnetic moments to a predetermined configuration, and thereby accelerate convergence towards self-consistency. Their use in a perturbative context, however, remains very limited. Here we present a general methodological framework to achieve parametric control over the local spin moments at the linear-response level. Our strategy builds on the concept of Legendre transform to switch between various flavors of magnetic functionals, and to relate their second derivatives via simple linear-algebra operations. Thereby, we can address an arbitrary response function at the time-dependent DFT level of theory with optimal accuracy and minimal computational effort. In the low frequency limit, we identify the leading correction to the existing adiabatic formulation of the problem [S. Ren \emph{et al.}, Phys. Rev. X {\bf 14}, 011041 (2024)], consisting in a renormalization of the phonon and magnon masses due to electron inertia. As a demonstration, we apply our methodology to the study of the THz optical response in bulk CrI3_3, where we identify a hybrid electromagnon with mixed spin-lattice character.
Born dynamical charges (Zdyn\textbf{Z}^\text{dyn}) play a key role in the lattice dynamics of most crystals, including both insulators and metals in the nonadiabatic ("clean") regime. Very recently, the so-called static Born charges, Zstat\textbf{Z}^\text{stat}, were introduced [G. Marchese, et al., Nat. Phys. 20\mathbf{20}, 88 (2024)] as a means to modeling the long-wavelength behavior of polar phonons in overdamped ("dirty") metals. Here we present a method to calculate Zstat\textbf{Z}^\text{stat} directly at the zone center, by applying the 2n+12n+1 theorem to the long-wavelength expansion of the charge response to a phonon. Furthermore, we relate Zstat\textbf{Z}^\text{stat} to the charge response to a uniform strain perturbation via an exact sum rule, where the quantum capacitance of the material plays a crucial role. We showcase our findings via extensive numerical tests on simple metals aluminum and copper, polar metal LiOsO3_3, and doped semiconductor SrTiO3_3. Based on our results, we critically discuss the physical significance of Zstat\textbf{Z}^\text{stat} in light of their dependence on the choice of the electrostatic reference, and on the length scale that is assumed in the definition of the macroscopic potentials.
Recent works have pointed out some worrisome inconsistencies in linear-response calculations performed with nonlocal pseudopotentials. Here we show that most of these issues are fixed by correctly adapting the pseudopotential to the motion of the corresponding nucleus, with a velocity dependence of the nonlocal operator. This prescription restores the correct Galilean covariance of the Schr\"odinger equation, and the expected identity between mechanical rototranslations and electromagnetic perturbations. We demonstrate our arguments by relating the interatomic force constants to the electromagnetic susceptibility of the system via a set of exact sum rules. Among other virtues, these results conclusively reconcile the inertial and electrical definitions of the Drude weight in metals.
We study quantum enhancement of sensitivity using squeezed light in a multi-parameter quantum sensor, the hybrid rf-dc optically pumped magnetometer (hOPM) [Phys. Rev. Applied 21, 034054, (2024)]. Using a single spin ensemble, the hOPM acquires both the dc field strength (scalar magnetometry), and resonantly detects one quadrature of the ac magnetic field at a chosen frequency (rf magnetometry). In contrast to the Bell-Bloom scalar magnetometer (BBOPM) [Phys. Rev. Lett. 127, 193601 (2021)], the back-action evasion in the hOPM is incomplete, leading to a complex interplay of the three quantum noise sources in this system: photon shot noise, spin projection noise, and measurement back-action noise. We observe these interactions using squeezed light as a tool to control the distribution of optical quantum noise between S2S_2 and S3S_3 polarization Stokes components, and the resulting effect on readout quantum noise and measurement back-action.
We investigate the accuracy of Eulerian perturbation theory for describing the matter and galaxy power spectra in real and redshift space in light of future observational probes for precision cosmology. Comparing the analytical results with a large suite of N-body simulations (160 independent boxes of 13.8 (Gpc/h)^3 volume each, which are publicly available), we find that re-summing terms in the standard perturbative approach predicts the real-space matter power spectrum with an accuracy of < 2% for k < 0.20 h/Mpc at redshifts z < 1.5. This is obtained following the widespread technique of writing the resummed propagator in terms of 1-loop contributions. We show that the accuracy of this scheme increases by considering higher-order terms in the resummed propagator. By combining resummed perturbation theories with several models for the mappings from real to redshift space discussed in the literature, the multipoles of the dark-matter power spectrum can be described with sub-percent deviations from N-body results for k < 0.15h/Mpc at z < 1. As a consequence, the logarithmic growth rate, f, can be recovered with sub-percent accuracy on these scales. Extending the models to massive dark-matter haloes in redshift space, our results describe the monopole term from N-body data within 2% accuracy for scales k < 0.15 h/Mpc at z < 0.5; here f can be recovered within < 5% when the halo bias is known. We conclude that these techniques are suitable to extract cosmological information from future galaxy surveys.
Parameter estimation is of fundamental importance in areas from atomic spectroscopy and atomic clocks to gravitational wave detection. Entangled probes provide a significant precision gain over classical strategies in the absence of noise. However, recent results seem to indicate that any small amount of realistic noise restricts the advantage of quantum strategies to an improvement by at most a multiplicative constant. Here, we identify a relevant scenario in which one can overcome this restriction and attain superclassical precision scaling even in the presence of uncorrelated noise. We show that precision can be significantly enhanced when the noise is concentrated along some spatial direction, while the Hamiltonian governing the evolution which depends on the parameter to be estimated can be engineered to point along a different direction. In the case of perpendicular orientation, we find superclassical scaling and identify a state which achieves the optimum.
We consider reversible work extraction from identical quantum batteries. From an ensemble of individually passive states, work can be produced only via global unitary (and thus entangling) operations. However, we show here that there always exists a method to extract all possible work without creating any entanglement, at the price of generically requiring more operations (i.e. additional time). We then study faster methods to extract work and provide a quantitative relation between the amount of generated multipartite entanglement and extractable work. Our results suggest a general relation between entanglement generation and the power of work extraction.
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