Erbium ($\text{Er}^{3+}$) emitters are relevant for optical applications due to their narrow emission line directly in the telecom C-band due to the ${}^\text{4}\text{I}_{\text{13/2}}$ $\rightarrow$ ${}^\text{4}\text{I}_{\text{15/2}}$ transition at 1.54 $\mu$m. Additionally they are promising candidates for future quantum technologies when embedded in thin-film silicon-on-insulator (SOI) to achieve fabrication scalability and CMOS compatibility. In this paper we integrate $\text{Er}^{3+}$ emitters in SOI metasurfaces made of closely spaced array of nanodisks, to study their spontaneous emission via room and cryogenic temperature confocal microscopy, off-resonance and in-resonance photoluminescence excitation at room temperature and time resolved spectroscopy. This work demonstrates the possibility to adopt CMOS-compatible and fabrication scalable metasurfaces for controlling and improving the collection efficiency of the spontaneous emission from the $\text{Er}^{3+}$ transition in SOI and could be adopted in similar technologically advanced materials.

Applying quantum computing in the computer-aided engineering (CAE) problems are highly expected since quantum computers yield potential exponential speedups for the operations between extremely large matrices and vectors. Although efficient quantum algorithms for the above problems have been intensively investigated, it remains a crucial task to extract all the grid-point values encoded in the prepared quantum states, which was believed to eliminate the achieved quantum advantage. In this paper, we propose a quantum-classical hybrid Fourier space readout (FSR) method to efficiently recover the underlying function from its corresponding quantum state. We provide explicit quantum circuits, followed by theoretical and numerical discussions on its complexity. In particular, the complexity on quantum computers has only a logarithmic dependence on the grid number, while the complexity on classical computers has a linear dependence on the number of target points instead of the grid number. Our result implies that the achieved quantum speedups are not necessarily ruined when we read out the solutions to the CAE problems.

This study explores the use of equivariant quantum neural networks (QNN) for generating molecular force fields, focusing on the rMD17 dataset. We consider a QNN architecture based on previous research and point out shortcomings in the parametrization of the atomic environments. These shortcomings limit its expressivity as an interatomic potential and precludes transferability between molecules. We propose a revised QNN architecture that addresses these shortcomings. While both QNNs show promise in force prediction, with the revised architecture showing improved accuracy, they struggle with energy prediction. Further, both QNNs architectures fail to demonstrate a meaningful scaling law of decreasing errors with increasing training data. These findings highlight the challenges of scaling QNNs for complex molecular systems and emphasize the need for improved encoding strategies, regularization techniques, and hybrid quantum-classical approaches.

In this study, we employed Fourier-based quantum phase estimation (QPE) to calculate X-ray absorption spectroscopy (XAS) spectra. The primary focus of this study is the calculation of the XAS spectra of transition metal $L_{2,3}$-edges, which are dominated by strong correlation effects. First, the Fe $L_{2,3}$-edge X-ray absorption near-edge structure of FePO$_4$ is calculated using a noiseless simulator. The present computation involves a comparison of three types of input states: a uniform superposition state, optimal entangled input state, and Slater function state. Subsequently, we investigated the resolution error of the QPE and statistical error attributed to the measurements. It was revealed that post-processing to introduce Lorentzian broadening reduces the statistical error, which becomes a significant problem for a large number of qubits. Subsequently, we implemented QPE on a trapped-ion quantum computer, encompassing three orbitals within the active space. To this end, we implemented QPE using dynamic circuits to reduce ancilla qubits and [[k+2, k, 2]] quantum error detection code to mitigate the quantum noise inherent in current quantum computers. As a result, it was demonstrated that hardware noise was reduced, and spectra close to the noiseless ones were obtained.

In this article, we compare the methods implementing the real-time evolution operator generated by a unitary diagonal matrix where its entries obey a known underlying real function. When the size of the unitary diagonal matrix is small, a well-known method based on Walsh operators gives a good and precise implementation. In contrast, as the number of qubits grows, the precise one uses exponentially increasing resources, and we need an efficient implementation based on suitable approximate functions. Using piecewise polynomial approximation of the function, we summarize the methods with different polynomial degrees. Moreover, we obtain the overheads of gate count for different methods concerning the error bound and grid parameter (number of qubits). This enables us to analytically find a relatively good method as long as the underlying function, the error bound, and the grid parameter are given. This study contributes to the problem of encoding a known function in the phase factor, which plays a crucial role in many quantum algorithms/subroutines. In particular, we apply our methods to implement the real-time evolution operator for the potential part in the first-quantized Hamiltonian simulation and estimate the resources (gate count and ancillary qubits) regarding the error bound, which indicates that the error coming from the approximation of the potential function is not negligible compared to the error from the Trotter-Suzuki formula.

Diamond is a promising platform for quantum information processing as it can host highly coherent qubits that could allow for the construction of large quantum registers. A prerequisite for such devices is a coherent interaction between nitrogen vacancy (NV) electron spins. Entanglement between dipolar-coupled NV spin pairs has been demonstrated, but with a limited entanglement fidelity and its error sources have not been characterized. Here, we design and implement a robust, easy to implement entangling gate between NV spins in diamond and quantify the influence of multiple error sources on the gate performance. Experimentally, we demonstrate a record gate fidelity of $F=(96.0 \pm 2.5)$ % under ambient conditions. Our identification of the dominant errors paves the way towards NV-NV gates beyond the error correction threshold.

Magnetic imaging with nitrogen-vacancy centers in diamond, also known as quantum diamond microscopy, has emerged as a useful technique for the spatial mapping of charge currents in solid-state devices. In this work, we investigate an application to photovoltaic (PV) devices, where the currents are induced by light. We develop a widefield nitrogen-vacancy microscope that allows independent stimulus and measurement of the PV device, and test our system on a range of prototype crystalline silicon PV devices. We first demonstrate micrometer-scale vector magnetic field imaging of custom PV devices illuminated by a focused laser spot, revealing the internal current paths in both short-circuit and open-circuit conditions. We then demonstrate time-resolved imaging of photocurrents in an interdigitated back-contact solar cell, detecting current build-up and subsequent decay near the illumination point with microsecond resolution. This work presents a versatile and accessible analysis platform that may find distinct application in research on emerging PV technologies.

Coupling microwave cavity modes with spin qubit transitions is crucial for enabling efficient qubit readout and control, long-distance qubit coupling, quantum memory implementation, and entanglement generation. We experimentally observe the coupling of different spin qubit transitions in Silicon Carbide (SiC) material to a 3D microwave (MW resonator mode around 12.6~GHz at a temperature of 10~mK. Tuning the spin resonances across the cavity resonance via magnetic-field sweeps, we perform MW cavity transmission measurements. We observe spin transitions of different spin defects that are detuned from each other by around 60-70~MHz. By optically exciting the SiC sample placed in the MW cavity with an 810~nm laser, we observe the coupling of an additional spin resonance to the MW cavity, also detuned by around 60-70 MHz from the centre resonance. We perform complementary confocal optical spectroscopy as a function of temperature from 4~K to 200~K. Combining the confocal spectroscopy results and a detailed analysis of the MW-resonator-based experiments, we attribute the spin resonances to three different paramagnetic defects: positively-charged carbon antisite vacancy pair (CAV$^+$), and the negatively-charged silicon vacancy spins located at two different lattice sites, namely V$_1$ and V$_2$ spins. The V$_1$ and V$_2$ lines in SiC are interesting qubit transitions since they are known to be robust to decoherence. Additionally, the CAV$^+$-transition is known to be a bright single-photon source. Consequently, the demonstration of the joint coupling of these spin qubits to a MW cavity mode could lead to interesting new modalities: The microwave cavity could act as an information bus and mediate long-range coupling between the spins, with potential applications in quantum computing and quantum communication, which is an attractive proposition in a CMOS-compatible material such as SiC.

The spectral characterization of quantum emitter luminescence over broad wavelength ranges and fast timescales is important for applications ranging from biophysics to quantum technologies. Here we present the application of time-domain Fourier transform spectroscopy, based on a compact and stable birefringent interferometer coupled to low-dark-count superconducting single-photon detectors, to the study of quantum emitters. We experimentally demonstrate that the system enables spectroscopy of quantum emitters over a broad wavelength interval from the near-infrared to the telecom range, where grating-based spectrometers coupled to InGaAs cameras are typically noisy and inefficient. We further show that the high temporal resolution of single-photon detectors, which can be on the order of tens of picoseconds, enables the monitoring of spin-dependent spectral changes on sub-nanosecond timescales.

NanoTerasu, a new 3 GeV synchrotron light source in Japan, began user operation in April 2024. It provides high-brilliance soft to tender X-rays and covers a wide spectral range from ultraviolet to tender X-rays. Its compact storage ring with a circumference of 349 m is based on a four-bend achromat lattice to provide two straight sections in each cell for insertion devices with a natural horizontal emittance of 1.14 nm rad, which is small enough for soft X-rays users. The NanoTerasu accelerator incorporates several innovative technologies, including a full-energy injector C-band linear accelerator with a length of 110 m, an in-vacuum off-axis injection system, a four-bend achromat with B-Q combined bending magnets, and a TM020 mode accelerating cavity with built-in higher-order-mode dampers in the storage ring. This paper presents the accelerator machine commissioning over a half-year period and our model-consistent ring optics correction. The first user operation with a stored beam current of 160 mA is also reported. We summarize the storage ring parameters obtained from the commissioning. This is helpful for estimating the effective optical properties of synchrotron radiation at NanoTerasu.

JT-60SA is a large superconducting tokamak built in Naka, Japan. After the successful achievement of its first MA-class plasma, the installation of several additional sub-systems, including a set of non-axisymmetric Error Field Correction Coils (EFCC), is ongoing. Optimization of future JT-60SA plasma scenarios will critically depend on the correct use of EFCC, including careful fulfillment of system specifications. In addition to that, preparation and risk mitigation of early ITER operations will greatly benefit from the experience gained by early EFCC application to JT-60SA experiments, in particular to optimize error field detection and control strategies. In this work, EFCC application in JT-60SA Initial Research Phase I perspective scenarios is modeled including plasma response. Impact of (Resonant) Magnetic Perturbations on the different plasma scenarios is assessed for both core and pedestal regions by the linear resistive MHD code MARS-F. The dominant core response to EFs is discussed case by case and compared to mode locking thresholds from literature. Typical current/voltage amplitudes and wave-forms are then compared to EFCC specifications in order to assess a safe operational space.

Gamma rays selectively interact with nuclei, induce and mediate nuclear reactions and elementary particle interactions, and exceed x-rays in penetrating power and thus are indispensable for analysis and modification of dense objects. Yet, the available gamma sources lack sufficient power and brightness. The predicted and highly desirable laser-driven gamma flash, from here on termed "Gamma Flash", based on inverse Compton scattering from solid targets at extreme irradiances (>$10^{23}W/cm^2$), would be the highest-power and the brightest terrestrial gamma source with a 30-40% laser-to-gamma energy conversion. However, Gamma Flash remains inaccessible experimentally due to the Bremsstrahlung background. Here we experimentally demonstrate a new interaction regime at the highest effective irradiance where Gamma Flash scaled quickly with the laser power and produced several times the number of Bremsstrahlung photons. Simulations revealed an attosecond, Terawatt Gamma Flash with a nanometre source size achieving a record brightness exceeding $~10^{23}photons/mm^2mrad^2s$ per 0.1% bandwidth at tens of MeV photon energies, surpassing astrophysical Gamma Ray Bursts. These findings could revolutionize inertial fusion energy by enabling unprecedented sub-micrometre/femtosecond resolution radiography of fuel mixing instabilities in extremely-compressed targets. The new gamma source could facilitate significant advances in time-resolved nuclear physics, homeland security, nuclear waste management and non-proliferation, while opening possibilities for spatially-coherent gamma rays.

The negatively-charged silicon vacancy center ($\rm V_{Si}^-$) in silicon carbide (SiC) is an emerging color center for quantum technology covering quantum sensing, communication, and computing. Yet, limited information currently available on the internal spin-optical dynamics of these color centers prevents us achieving the optimal operation conditions and reaching the maximum performance especially when integrated within quantum photonics. Here, we establish all the relevant intrinsic spin dynamics of negatively charged $\rm V_{Si}^-$ center in 4H-SiC by an in-depth electronic fine structure modeling including intersystem-crossing and deshelving mechanisms. With carefully designed spin-dependent measurements, we obtain all previously unknown spin-selective radiative and non-radiative decay rates. To showcase the relevance of our work for integrated quantum photonics, we use the obtained rates to propose a realistic implementation of time-bin entangled multi-photon GHZ and cluster state generation. We find that up to 3-photon GHZ/cluster states are readily within reach using the existing nanophotonic cavity technology.

Accurate measurements of alternating current (AC) and direct current(DC) ratios are fundamental to electric power metrology. However, conventional current comparators for AC and DC typically rely on distinct technologies-electromagnetic induction for AC and superconducting quantum interference devices for DC. This technological divide leads to a fragmented and complex traceability system. Bridging this gap is critical for developing unified current standards that meet the demands of emerging power technologies. In this work, we present a compact, room-temperature AC/DC current comparator that integrates a diamond-based magnetometer using nitrogen-vacancy centers. The device achieves an accuracy of 10-8 for both AC and DC signals and supports a system bandwidth up to 300 Hz, without the need for cryogenics. It surpasses the performance of typical AC comparators, offering ten-fold higher accuracy, and matches that of state-of-the-art DC comparators. This unified, cryogenics-free solution not only enhances precision and versatility but also expands the applicability of the system to DC resistance bridges in quantum electrical standards.

One of the crucial generic techniques for quantum computation is amplitude encoding. Although several approaches have been proposed, each of them often requires exponential classical-computational cost or an oracle whose explicit construction is not provided. Given the growing demands for practical quantum computation, we develop moderately specialized encoding techniques that generate an arbitrary linear combination of localized complex functions. We demonstrate that $n_{\mathrm{loc}}$ discrete Lorentzian functions as an expansion basis set lead to eficient probabilistic encoding, whose computational time is $\mathcal{O}( \max ( n_{\mathrm{loc}}^2 \log n_{\mathrm{loc}},n_{\mathrm{loc}}^2 \log n_q, n_q ))$ for $n_q$ data qubits equipped with $\log_2 n_{\mathrm{loc}}$ ancillae. Furthermore, amplitude amplification in combination with amplitude reduction renders it deterministic analytically with controllable errors and the computational time is reduced to $\mathcal{O}( \max ( n_{\mathrm{loc}}^{3/2} \log n_{\mathrm{loc}}, n_{\mathrm{loc}}^{3/2} \log n_q, n_q )).$ We estimate required resources for applying our scheme to quantum chemistry in real space. We also show the results on real superconducting quantum computers to confirm the validity of our techniques.

Magnetometry with nitrogen-vacancy (NV) centers has so far been measured via emission of light from NV centers or via absorption at the singlet transition at 1042 nm. Here, we demonstrate a phenomenon of broadband optical absorption by the NV centers starting in the emission wavelength and reaching up to 1000 nm. The measurements are enabled by a high-finesse cavity, which is used for room temperature continuous wave pump-probe experiments. The red to infrared probe beam shows the typical optically detected magnetic resonance (ODMR) signal of the NV spin with contrasts up to 42 %. This broadband optical absorption is not yet reported in terms of NV magnetometry. We argue that the lower level of the absorbing transition could be the energetically lower NV singlet state, based on the increased optical absorption for a resonant microwave field and the spectral behavior. Investigations of the photon-shot-noise-limited sensitivity show improvements with increasing probe wavelength, reaching an optimum of 7.5 pT/$\sqrt{\mathrm{Hz}}$. The results show significantly improved ODMR contrast compared to emission-based magnetometry. This opens a new detection wavelength regime with coherent laser signal detection for high-sensitivity NV magnetometry.

Kagome superconductors AV3Sb5 (A = K, Rb, Cs) exhibit a characteristic superconducting and charge-density wave (CDW) phase diagram upon carrier doping and chemical substitution. However, the key electronic states responsible for such a phase diagram have yet to be clarified. Here we report a systematic micro-focused angle-resolved photoemission spectroscopy (ARPES) study of Cs(V1-xCrx)3Sb5 as a function of Cr content x, where Cr substitution causes monotonic reduction of superconducting and CDW transition temperatures. We found that the V-derived bands forming saddle points at the M point and Dirac nodes along high-symmetry cuts show an energy shift due to electron doping by Cr substitution, whereas the Sb-derived electron band at the Gamma point remains almost unchanged, signifying an orbital-selective band shift. We also found that band doubling associated with the emergence of three-dimensional CDW identified at x = 0 vanishes at x = 0.25, in line with the disappearance of CDW. A comparison of band diagrams among Ti-, Nb-, and Cr-substituted Cs(V1-xCrx)3Sb5 suggests the importance to simultaneously take into account the two saddle points at the M point and their proximity to the Fermi energy, to understand the complex phase diagram against carrier doping and chemical pressure.

A compact energy-recovery linac (cERL) has been un-der construction at KEK since 2009 to develop key technologies for the energy-recovery linac. The cERL began operating in 2013 to create a high-current beam with a low-emittance beam with stable continuous wave (CW) superconducting cavities. Owing to the development of critical components, such as the DC gun, superconducting cavities, and the design of ideal beam transport optics, we have successfully established approximately 1 mA stable CW operation with a small beam emittance and extremely small beam loss. This study presents the details of our key technologies and experimental results for achieving 100% energy recovery operation with extremely small beam loss during a stable, approximately 1 mA CW beam operation.