National Laboratory of Solid-State Microstructures
The MnBi2_2Te4_4 material family has emerged as a key platform for exploring magnetic topological phases, most notably exemplified by the experimental realization of the axion insulator state. While spin dynamics are known to significantly influence the axion state, a profound understanding of their interplay remains elusive. In this work, we employ an antiferromagnetic spin-chain model to demonstrate that an external magnetic field induces extrinsic perpendicular magnetic anisotropy. We find that an in-plane field stabilizes the antiferromagnetic order, whereas an out-of-plane field destabilizes it and triggers spin-flop transitions. Remarkably, near the surface spin-flop transition in even-layer MnBi2_2Te4_4 films, the axion insulator state undergoes a sharp switching behavior accompanied by distinct magnetoelectric responses. Furthermore, we propose that this switchable axionic magnetoelectric effect can be utilized to convert alternating magnetic field signals into measurable square-wave magneto-optical outputs, thereby realizing an axionic analog of a zero-crossing detector. Our findings could open a pathway toward potential applications of axion insulators in next-generation spintronic devices.
Revealing the momentum-resolved electronic structure of infinite-layer nickelates is essential for understanding this new class of unconventional superconductors, but has been hindered by the formidable challenges in improving the sample quality. In this work, we report for the first time the angle-resolved photoemission spectroscopy of superconducting La0.8_{0.8}Sr0.2_{0.2}NiO2_{2} films prepared by molecular beam epitaxy and in situ{\mathrm{\textit{in situ}}} atomic-hydrogen reduction. The measured Fermi topology closely matches theoretical calculations, showing a large Ni-dx2y2d_{x^2-y^2} derived Fermi sheet that evolves from hole-like to electron-like along kzk_{z}, and a three-dimensional (3D) electron pocket centered at Brillouin zone corner. The Ni-dx2y2d_{x^2-y^2} derived bands show a mass enhancement (m/mDFTm^*/m_{\rm{DFT}}) of 2-3,while the 3D electron band shows negligible band renormalization. Moreover, the Ni-dx2y2d_{x^2-y^2} derived states also display a band dispersion anomaly at higher binding energy, reminiscent of the waterfall feature and kinks observed in cuprates.
Moiré transition metal dichalcogenide (TMD) systems provide a tunable platform for studying electron-correlation driven quantum phases. Such phases have so far been found at rational fillings of the moiré superlattice, and it is believed that lattice commensurability plays a key role in their stability. In this work, we show via magnetotransport measurements on twisted WSe2 that new correlated electronic phases can exist away from commensurability. The first phase is an antiferromagnetic metal that is driven by proximity to the van Hove singularity. The second is a re-entrant magnetic field-driven insulator. This insulator is formed from a small and equal density of electrons and holes with opposite spin projections - an Ising excitonic insulator.
Transformer neural networks, known for their ability to recognize complex patterns in high-dimensional data, offer a promising framework for capturing many-body correlations in quantum systems. We employ an adapted Vision Transformer (ViT) architecture to model quantum impurity models, optimizing it with a subspace expansion scheme that surpasses conventional variational Monte Carlo in both accuracy and efficiency. Benchmarks against matrix product states in single- and three-orbital Anderson impurity models show that these ViT-based neural quantum states achieve comparable or superior accuracy with significantly fewer variational parameters. We further extend our approach to compute dynamical quantities by constructing a restricted excitation space that effectively captures relevant physical processes, yielding accurate core-level X-ray absorption spectra. These findings highlight the potential of ViT-based neural quantum states for accurate and efficient modeling of quantum impurity models.
Two-photon Hong-Ou-Mandel (HOM) interference is a fundamental quantum effect with no classical counterpart. The exiting researches on two-photon interference were mainly limited in one degree of freedom (DoF), hence it is still a challenge to realize the quantum interference in multiple DoFs. Here we demonstrate the HOM interference between two hyper-entangled photons in two DoFs of polarization and orbital angular momentum (OAM) for all the sixteen hyper-entangled Bell states. We observe hyper-entangled two-photon interference with bunching effect for ten symmetric states (nine Boson-Boson states, one Fermion-Fermion state) and anti-bunching effect for six anti-symmetric states (three Boson-Fermion states, three Fermion-Boson states). More interestingly, expanding the Hilbert space by introducing an extra DoF for two photons enables to transfer the unmeasurable external phase in the initial DoF to a measurable internal phase in the expanded two DoFs. We directly measured the symmetric exchange phases being 0.012±0.0020.012 \pm 0.002, 0.025±0.0020.025 \pm 0.002 and 0.027±0.0020.027 \pm 0.002 in radian for the three Boson states in OAM and the anti-symmetric exchange phase being 0.991π±0.0020.991 \pi \pm 0.002 in radian for the other Fermion state, as theoretical predictions. Our work may not only pave the way for more wide applications of quantum interference, but also develop new technologies by expanding Hilbert space in more DoFs.
Federated learning is essential for decentralized, privacy-preserving model training in the data-driven era. Quantum-enhanced federated learning leverages quantum resources to address privacy and scalability challenges, offering security and efficiency advantages beyond classical methods. However, practical and scalable frameworks addressing privacy concerns in the quantum computing era remain undeveloped. Here, we propose a practical quantum federated learning framework on quantum networks, utilizing distributed quantum secret keys to protect local model updates and enable secure aggregation with information-theoretic security. We experimentally validate our framework on a 4-client quantum network with a scalable structure. Extensive numerical experiments on both quantum and classical datasets show that adding a quantum client significantly enhances the trained global model's ability to classify multipartite entangled and non-stabilizer quantum datasets. Simulations further demonstrate scalability to 200 clients with classical models trained on the MNIST dataset, reducing communication costs by 75%75\% through advanced model compression techniques and achieving rapid training convergence. Our work provides critical insights for building scalable, efficient, and quantum-secure machine learning systems for the coming quantum internet era.
The quantum geometric tensor (QGT) fundamentally encodes the geometry and topology of quantum states in both Hermitian and non-Hermitian regimes. While adiabatic perturbation theory links its real part (quantum metric) and imaginary part (Berry curvature) to energy fluctuations and generalized forces, respectively, in Hermitian systems, direct measurement of the QGT, which defined using both left and right eigenstates of non-Hermitian Hamiltonian, remains challenging. Here we develop two quantum simulation schemes to directly extract all components of the QGT in pseudo-Hermitian systems with real spectra. Each scheme independently determines the complete QGT using generalized expectation values of either the energy fluctuation operator or the generalized force operator with respect to two time-evolved states prepared through distinct nonadiabatic evolutions, thereby establishing two self-contained measurement protocols. We illustrate the validity of these schemes on two qq-deformed 2-band models: one with nontrivial topology, and the other with a nonvanishing off-diagonal quantum metric. Numerical simulations show that both schemes achieve high-fidelity agreement with theoretical predictions for measuring the QGT of both models, and successfully capture the topological phase transition of the first model using Chern numbers calculated from Berry curvatures. This work provides a framework for extending dynamical measurement schemes from Hermitian to pseudo-Hermitian systems with real spectra.
Topological nodal superconductors (SCs) have attracted considerable interest due to their gapless bulk excitations and exotic surface states. In this paper, by establishing a general framework of the effective theory for multi-orbital SCs, we realize a class of three-dimensional (3D) time-reversal (T )-invariant Dirac SCs, with their topologically protected gapless Dirac nodes being located at general positions in the Brillouin zone. By introducing T -breaking pairing perturbations, we demonstrate the existence of Majorana hinge modes in these Dirac SCs as evidence of their realization of higher-order topology. We also propose a new kind of T -breaking Dirac SCs, whose Dirac nodes possess nonzero even chiralities and so are characterized by surface Majorana arcs.
Quantum entanglement -- correlations of particles that are stronger than any classical analogue -- is the basis for research on the foundations of quantum mechanics and for practical applications such as quantum networks. Traditionally, entanglement is achieved through local interactions or via entanglement swapping, where entanglement at a distance is generated through previously established entanglement and Bell-state measurements. However, the precise requirements enabling the generation of quantum entanglement without traditional local interactions remain less explored. Here we demonstrate that independent particles can be entangled without the need for direct interaction, prior established entanglement, or Bell-state measurements, by exploiting the indistinguishability of the origins of photon pairs. Our demonstrations challenge the long-standing belief that the prior generation and measurement of entanglement are necessary prerequisites for generating entanglement between independent particles that do not share a common past. In addition to its foundational interest, we show that this technique might lower the resource requirements in quantum networks, by reducing the complexity of photon sources and the overhead photon numbers.
A typical imaging scenario requires three basic ingredients: 1. a light source that emits light, which in turn interacts and scatters off the object of interest; 2. detection of the light being scattered from the object and 3. a detector with spatial resolution. These indispensable ingredients in typical imaging scenarios may limit their applicability in the imaging of biological or other sensitive specimens due to unavailable photon-starved detection capabilities and inevitable damage induced by interaction. Here, we propose and experimentally realize a quantum imaging protocol that alleviates all three requirements. By embedding a single-photon Michelson interferometer into a nonlinear interferometer based on induced coherence and harnessing single-pixel imaging technique, we demonstrate interaction-free, single-pixel quantum imaging of a structured object with undetected photons. Thereby, we push the capability of quantum imaging to the extreme point in which no interaction is required between object and photons and the detection requirement is greatly reduced. Our work paves the path for applications in characterizing delicate samples with single-pixel imaging at silicon-detectable wavelengths.
We elaborate the first theoretical realization of two dimensional itinerant topological magnons, based on the quarter filled Haldane-Hubbard model with a nearly-flat electron band. By using the exact diagonalization method with a projection onto this band, we obtain the spin wave excitations over the itinerant ferromagnetic ground state. In the flatband limit, the excitation exhibits similar dispersion to the free electron band with Dirac magnons. The nonflatness of the electron band opens a topological gap at Dirac points and leads to an acoustic magnon band with a nonzero Chern number. We further show that tuning the sublattice Hubbard interactions or the next-nearest-neighbor hopping can induce a topological transition characterized by the gap closing and reopening, and the existence of the in-gap magnons on magnetic domain walls. We find an exact set of bases for magnons in the flatband limit constructed from sublattice particle-hole vectors and derive an effective model to explore the origin of the topological magnon which is attributed to the ``mass inversion mechanism''.
Twisted transition metal dichalcogenides (tTMDs) provide a highly tunable platform to explore the interplay between strong correlation and topology. Among them, the properties involving the charge degree of freedom have been extensively studied, while those related to spin are much less investigated. Motivated by the recent discovery of integer and fractional quantum anomalous Hall effects in tMoTe2_2, where the flat-band ferromagnetism is one of the essential prerequisites, we investigate theoretically the spin excitations out of the flat-band ferromagnetic ground state in tMoTe2_2. Remarkably, we identify the itinerant magnons and spin excitons with nontrivial topology. We elaborate that the topology of these itinerant spin excitations, which are described as particle-hole bound states, inherits directly from that of the underlying electrons and is essentially different from that in local spin systems. Thus, we establish a direct relationship of the topology between the many-body excitations and their fundamental constituents. We further demonstrate that by tuning the displacement field, a topological transition for both the magnon and spin exciton happens, leading to a step-like change and bifurcation in the thermal Hall conductance, which could serve as unique and compelling evidence to be tested experimentally.
Cells not only can be motile by crawling but are also capable of non-motility active motions like periodic contraction or pulsation. In this work, based on a Voronoi cell model, we show how this non-motility activity affects the structure, dynamic and density fluctuations of cellular monolayers. Our model shows that random cell pulsation fluidizes solid epithelial tissues into a hyperuniform fluid state, while pulsation synchronization inhibits the fluidity and causes a reverse solidification. Our results indicate this solidification is a BKT-type transition, characterized by strong density/dynamic heterogeneity arising from the annihilation of topological defects in the pulsating phase space. The magnitude and length scale of density heterogeneity diverge with the pulsating period, resulting in an opposite giant density fluctuation or anti-hyperuniformity. We propose a fluctuating hydrodynamic theory that can unify the two opposite anomalous fluctuation phenomena. Our findings can help to understand recent experimental observations in MDCK monolayer.
Skyrmions--topologically protected nanoscale spin textures with vortex-like configurations--hold transformative potential for ultra-dense data storage, spintronics and quantum computing. However, their practical utility is challenged by dynamic instability, complex interaction, and the lack of deterministic control. While recent efforts using classical wave systems have enabled skyrmion simulations via engineered excitations, these realizations rely on fragile interference patterns, precluding stable transport and flexible control. Here, we introduce a skyrmion molecule lattice, a novel architecture where pairs of spin skyrmions with opposite polarizability are symmetry-locked into stable molecule configurations. These molecules emerge as propagating eigenstates of the system, overcoming the static limitations of previous realizations. We further develop a boundary engineering technique, achieving precise control over skyrmion creation, deformation, annihilation, and polarizability inversion. As a proof of concept, we design a graphene-like acoustic surface wave metamaterial, where meta-atom pairs generate vortices with opposite orbital angular momenta, which couple to acoustic spin textures, forming skyrmion molecules. Experimental measurements confirm their stable transport and flexible control. Our work leverages the symmetry-locked molecule lattice to preserve the topological quasiparticle nature of skyrmions, offering a universal framework for their stabilization, transportation and manipulation. This bridges critical gaps in skyrmion physics, with potential impacts on wave-based sensing, information processing, and topological waveguiding.
We investigate the spin-12\frac{1}{2} antiferromagnetic Heisenberg model with a Dzyaloshinskii-Moriya interaction on kagome lattice, making use of the variational Monte Carlo technique. An exotic quantum spin state is found to arise from a melting of the Q=0\boldsymbol{Q} = 0 long-range magnetic order by a topological transition, when a small anisotropic third nearest-neighbor antiferromagnetic Heisenberg interaction is turned on. This novel state is a gapped quantum spin liquid, characterized by a topological order with ground-state degeneracy ng=4n_g = 4 and topological entanglement entropy γ=ln2\gamma = \ln 2, suggesting it is an Abelian topological phase. Furthermore, the Chern numbers of the spin-up (-down) spinon occupied bands of this state are C=±1C_{\uparrow \downarrow} = \pm 1, respectively. From this perspective, this state is also a time-reversal symmetric (total Chern number Ctotal=0C_{total} = 0) topological insulator with spinons as the chiral edge states, which carry opposite spin and move in the opposite direction. It is analogous to the quantum spin Hall state but the spin current is carried by deconfined spinons in a quantum spin liquid, so is dubbed as the spinon quantum spin Hall state.
31 Jul 2025
While thin film lithium niobate (TFLN) is known for efficient signal generation, on-chip signal amplification remains challenging from fully integrated optical communication circuits. Here we demonstrate the continuous-wave-pump optical parametric amplification (OPA) using an x-cut domain-engineered TFLN waveguide, with high gain over the telecom band up to 13.9 dB, and test it for high signal-to-noise ratio signal amplification using a commercial optical communication module pair. Fabricated in wafer scale using common process as devices including modulators, this OPA device marks an important step in TFLN photonic integration.
When a quantum system evolves so that it returns to its initial state, it will acquire a geometric phase acting as a memory of the transformation of a physical system, which has been experimentally measured in a variety of physical systems. In optics, the most prominent example is the Pancharatnam-Berry (PB) phase. Recent technological advances in phase and polarization structure have led to the discovery of high-order PB phases with structured light fields. The study on the high-order PB phase is limited in the context of elementary quantum states of light, especially in the case of photon number states. Here, we experimentally investigate the differences of high-order PB phases between single-photon and N00N states. Our results show that the PB phase, like the dynamic phase, can also be doubled under two-photon states, which can greatly improve the phase sensitivity for greater NN in N00N states and high-order structured photons. This may show some implications for quantum precision measurement and quantum state engineering based on geometric phase.
Circularly polarized phonons offer a new route for mediating angular momentum in solids. However, controlling phonon angular momentum without altering the material's structure or composition remains challenging. Here, we demonstrate the non-volatile switching of angular momentum-carrying phonons by leveraging intrinsic ferrimagnetism in an insulator. We find a pair of chiral phonons with giant energy splitting reaching 20% of the phonon frequency, due to spontaneously broken time-reversal symmetry. With a moderate magnetic field, the phonon angular momentum of the two chiral phonon branches can be switched along with the magnetization. Notably, near the critical temperature, the effective phonon magnetic moment is enhanced, reaching 2.62 Bohr magneton, exceeding the moment of a magnon. A microscopic model based on phonon-magnon coupling accounts for the observations. Furthermore, we identify two types of phononic domains with opposite phonon Zeeman splitting and propose the existence of topologically protected phononic edge modes at domain boundaries. These results demonstrate effective manipulation of chiral phonons with magnetism, and pave the way for engineering chiral phononic domains on the micrometer scale.
A new module within the machine learning and graph theory assisted universal structure searcher (MAGUS) framework reliably predicts known surface reconstruction ground states, including the Si(100) asymmetric dimer and Si(111) DAS model, and identifies a novel low-energy surface for 4H-SiC in Si-rich environments. This work leverages machine learning potentials and specific mutation strategies to improve the efficiency and accuracy of surface structure searches.
A full-fledged quantum network relies on the formation of entangled links between remote location with the help of quantum repeaters. The famous Duan-Lukin-Cirac-Zoller quantum repeater protocol is based on long distance single-photon interference, which not only requires high phase stability but also cannot generate maximally entangled state. Here, we propose a quantum repeater protocol using the idea of post-matching, which retains the same efficiency as the single-photon interference protocol, reduces the phase-stability requirement and can generate maximally entangled state in principle. We also outline an implementation of our scheme based on the Kerr nonlinear resonator. Numerical simulations show that our protocol has its superiority by comparing with existing protocols under a generic noise model and show the feasibility of building a large-scale quantum communication network with our scheme. We believe our work represents a crucial step towards the construction of a fully-connected quantum network.
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