We present an analytical description of the tunneling dynamics between two coupled Bose-Einstein condensates in the Josephson regime. The model relies on the classical analogy with a rigid pendulum and focuses on two dynamical modes of this system: Josephson oscillations and Macroscopic Quantum Self-Trapping. The analogy is extended to include an energy difference between the two superfluids caused by an asymmetry in the trapping potential. The model is compatible with the mean-field predictions of the two-mode Bose-Hubbard model. It gives new insights on the mean-field model by involving experimentally measurable parameters with reduced correlations. For agreement with recent experimental observations, we establish heuristic formulas including a dissipation. We conclude with a convincing application of the model to several sets of experimental results.

Hybrid evolution protocols, composed of unitary dynamics and repeated, weak or projective measurements, give rise to new, intriguing quantum phenomena, including entanglement phase transitions and unconventional conformal invariance. Defying the complications imposed by the non-linear and stochastic nature of the measurement process, we introduce a scenario of measurement-induced many body evolution, which possesses an exact analytical solution: bosonic Gaussian measurements. The evolution features a competition between the continuous observation of linear boson operators and a free Hamiltonian, and it is characterized by a unique and exactly solvable covariance matrix. Within this framework, we then consider an elementary model for quantum criticality, the free boson conformal field theory, and investigate in which way criticality is modified under measurements. Depending on the measurement protocol, we distinguish three fundamental scenarios (a) enriched quantum criticality, characterized by a logarithmic entanglement growth with a floating prefactor, or the loss of criticality, indicated by an entanglement growth with either (b) an area-law or (c) a volume-law. For each scenario, we discuss the impact of imperfect measurements, which reduce the purity of the wavefunction and are equivalent to Markovian decoherence, and present a set of observables, e.g., real-space correlations, the relaxation time, and the entanglement structure, to classify the measurement-induced dynamics for both pure and mixed states. Finally, we present an experimental tomography scheme, which grants access to the density operator of the system by using the continuous measurement record only.

Optical Bloch equations and rate equations serve as powerful tools to model light-matter interactions from textbook-like two-level atoms to the complex internal dynamics of molecules. A particular challenge in this context is posed by molecular laser cooling, where many dozens or hundreds of levels need to be taken into account for a comprehensive modeling. Here, we present MoleCool, a numerically efficient Python toolbox to implement and solve the corresponding differential equation systems. We illustrate both the capabilities of the toolbox and some of the intricacies of molecular laser cooling by educational examples, which range from simple Rabi oscillations to spontaneous and coherent cooling schemes for various currently studied or considered molecular species. This includes, in particular, a comprehensive modeling of laser cooling dynamics with full hyperfine structure resolution in radioactive radium monofluoride (RaF), as well as studies of other complex species such as barium monofluoride (BaF) and ytterbium monohydroxide (YbOH).

The field of indefinite causal order has seen significant advancements in recent years. While classically the causal order of two timelike separated events A and B is fixed - either A before B or B before A - this is no longer true in quantum theory. There, it is possible to encounter superpositions of causal orders. The quantum switch is one of the most prominent processes with indefinite causal order. While the optical quantum switch has been successfully implemented in experiments, some argue that this merely simulates a process with indefinite causal order and that a superposition of spacetime metrics is required for a true realization. Here, we provide a relativistic definition of causal order, show that it encompasses both the optical and gravitational quantum switch, and does not differentiate between them. Moreover, we show that this notion of causal order is invariant under so-called quantum diffeomorphisms and that it is an operationally meaningful observable in both the general relativistic and quantum mechanical sense. Importantly, this observable does not distinguish between the indefinite causal order implemented in the optical and gravitational quantum switch, thus supporting the thesis that the optical quantum switch is just as much a realization of indefinite causal order as its gravitational counterpart.

Control of quantum systems typically relies on the interaction with electromagnetic radiation. In this study, we experimentally show that the electromagnetic near-field of a spatially modulated freespace electron beam can be used to drive spin systems, demonstrating free-electron-bound-electron resonant interaction. By periodically deflecting the electron beam of a scanning electron microscope in close proximity to a spin-active solid-state sample, and sweeping the deflection frequency across the spin resonance, we directly observe phase coherent coupling between the electron beam's nearfield and the two spin states. This method relies only on classically shaping the electron beams transversal correlations and has the potential to enable coherent control of quantum systems with unprecedented, electron microscopic resolution, opening novel possibilities for advanced spectroscopic tools in nanotechnology.

By integrating tweezer arrays with a high-cooperativity ring cavity with chiral atom-cavity coupling, we demonstrate highly directional Bragg scattering from a programmable number of atoms. Through accurate control of the interatomic distance, we observe a narrowing-down of the Bragg peak as we increase the atom number one by one. The observed high-contrast Bragg interference is enabled by cavity sideband cooling of both the radial and axial motions to near the ground state with phonon occupation numbers below 0.17 and 3.4, respectively. This new platform that integrates strong and controlled atom-light coupling into atomic arrays enables applications from programmable quantum optics to quantum metrology and computation.

We describe a deterministic and experimentally feasible protocol for generating entangled pairs of ultracold neutral atoms through controlled dissociation of diatomic Feshbach molecules. The dissociation process naturally produces nonlocal quantum correlations in spin, position-momentum, and path degrees of freedom, enabling the deterministic preparation of Einstein-Podolsky-Rosen pairs of massive particles and multiqubit states through hyperentangled encoding. Having each atom of the pair prepared in a matter waveguide, the scheme can be scaled to hundreds of parallel entanglement sources in an array connected to a matter wave optical network of beam splitters, phase shifters, interferometers, tunnel junctions and local detectors. The protocol builds on established techniques, including programmable optical potentials, high-fidelity single-particle control, single-molecule initialization, controlled molecular dissociation, and quantum gas microscopy with near-perfect detection, making it directly implementable with current technology. The proposed architecture naturally integrates with atomtronics circuits and chip-based matter-wave optics, offering a deterministic entanglement source for quantum nonlocality tests, precision metrology, and scalable neutral-atom quantum processors.

Emergent collective excitations constitute a hallmark of interacting quantum many-body systems, yet in solid-state platforms their study has been largely limited by the constraints of linear-response probes and by finite momentum resolution. We propose to overcome these limitations by combining the spatial resolution of ultracold atomic systems with the nonlinear probing capabilities of two-dimensional spectroscopy (2DS). As a concrete illustration, we analyze momentum-resolved 2DS of the quantum sine-Gordon model describing the low energy dynamics of two weakly coupled one-dimensional Bose-Einstein condensates. This approach reveals distinctive many-body signatures, most notably asymmetric cross-peaks reflecting the interplay between isolated ($B_2$ breather) and continuum ($B_1$ pair) modes. The protocol further enables direct characterization of anharmonicity and disorder, establishing momentum-resolved 2DS as both a powerful diagnostic for quantum simulators and a versatile probe of correlated quantum matter.

The structure of solids and their phases is mainly determined by static Coulomb forces while the coupling of charges to the dynamical, i.e., quantized degrees of freedom of the electromagnetic field plays only a secondary role. Recently, it has been speculated that this general rule can be overcome in the context of cavity quantum electrodynamics (QED), where the coupling of dipoles to a single field mode can be dramatically enhanced. Here we present a first exact analysis of the ground states of a dipolar cavity QED system in the non-perturbative coupling regime, where electrostatic and dynamical interactions play an equally important role. Specifically, we show how strong and long-range vacuum fluctuations modify the states of dipolar matter and induce novel phases with unusual properties. Beyond a purely fundamental interest, these general mechanisms can be important for potential applications, ranging from cavity-assisted chemistry to quantum technologies based on ultrastrongly coupled circuit QED systems.

Realizing a strong interaction between individual optical photons is an important objective of research in quantum science and technology. Since photons do not interact directly, this goal requires, e.g., an optical medium in which the light experiences a phase shift that depends nonlinearly on the photon number. Once the additional phase shift for two photons reaches pi, such an ultra-strong nonlinearity could even enable the direct implementation of high-fidelity quantum logic operations. However, the nonlinear response of standard optical media is many orders of magnitude too weak for this task. Here, we demonstrate the realization of an optical fiber-based nonlinearity that leads to an additional two-photon phase shift close to the ideal value of pi. Our scheme employs a whispering-gallery-mode resonator, interfaced by an optical nanofiber, where the presence of a single rubidium atom in the resonator results in a strongly nonlinear response. We experimentally show that this results in entanglement of initially independent incident photons. The demonstration of this ultra-strong nonlinearity in a fiber-integrated system is a decisive step towards scalable quantum logics with optical photons.

Computation is an input-output process, where a program encoding a problem to be solved is inserted into a machine that outputs a solution. Quantum computation conventionally relies on classical, external control outside the quantum computer to execute a program, obscuring computational and thermodynamic resources required. To understand the fundamental limits of computation, however, it is pivotal to work with a fully self-contained description of a quantum computation, modeling the resources on the same footing as the computation itself. By developing a framework that we dub the autonomous Quantum Processing Unit (aQPU) we model quantum computation in the framework of autonomous thermal machines. Consisting of an internal quantum timekeeping mechanism, instruction register and memory system the aQPU allows investigating relationships between thermodynamic cost, complexity, speed and fidelity of a desired quantum computation.

We demonstrate how a single heat exchange between a probe thermal qubit and multi-qubit thermal machine encoding a Boolean function, can determine whether the function is balanced or constant, thus providing a novel thermodynamic solution to the Deutsch-Jozsa problem. We introduce a thermodynamic model of quantum query complexity, showing how qubit thermal machines can act as oracles, queried via heat exchange with a probe. While the Deutsch-Jozsa problem requires an exponential encoding in the number of oracle bits, we also explore the Bernstein-Vazirani problem, which admits a linear thermal oracle and a single thermal query solution. We establish bounds on the number of samples needed to determine the probe temperature encoding the solution for the Deutsch-Jozsa problem, showing that it remains constant with problem size. Additionally, we propose a proof-of-principle experimental implementation to solve the 3-bit Bernstein-Vazirani problem via thermal kickback. This work bridges thermodynamics and complexity theory, suggesting a new test bed for quantum thermodynamic computing.

Transport properties play a crucial role in defining materials as insulators, metals, or superconductors. A fundamental parameter in this regard is the Drude weight, which quantify the ballistic transport of charge carriers. In this work, we measure the Drude weights of an ultracold gas of interacting bosonic atoms confined to one dimension, characterising the induced atomic and energy currents in response to perturbations with an external potential. We induce currents through two distinct experimental protocols; by applying a constant force to the gas, and by joining two subsystems prepared in different equilibrium states. By virtue of integrability, dynamics of the system is governed by ballistically propagating, long-lived quasi-particle excitations, whereby Drude weights almost fully characterise large-scale transport. Indeed, our results align with predictions from a recently developed hydrodynamic theory, demonstrating almost fully dissipationless transport, even at finite temperatures and interactions. These findings not only provide experimental validation of the hydrodynamic predictions but also offer methodologies applicable to various condensed matter systems, facilitating further studies on the transport properties of strongly correlated quantum matter.

Do the laws of quantum physics still hold for macroscopic objects - this is at the heart of Schrödinger's cat paradox - or do gravitation or yet unknown effects set a limit for massive particles? What is the fundamental relation between quantum physics and gravity? Ground-based experiments addressing these questions may soon face limitations due to limited free-fall times and the quality of vacuum and microgravity. The proposed mission MAQRO may overcome these limitations and allow addressing those fundamental questions. MAQRO harnesses recent developments in quantum optomechanics, high-mass matter-wave interferometry as well as state-of-the-art space technology to push macroscopic quantum experiments towards their ultimate performance limits and to open new horizons for applying quantum technology in space. The main scientific goal of MAQRO is to probe the vastly unexplored "quantum-classical" transition for increasingly massive objects, testing the predictions of quantum theory for truly macroscopic objects in a size and mass regime unachievable in ground-based experiments. The hardware for the mission will largely be based on available space technology. Here, we present the MAQRO proposal submitted in response to the (M4) Cosmic Vision call of the European Space Agency for a medium-size mission opportunity with a possible launch in 2025.

Control of quantum systems typically relies on the interaction with electromagnetic radiation. In this study, we experimentally show that the electromagnetic near-field of a spatially modulated freespace electron beam can be used to drive spin systems, demonstrating free-electron-bound-electron resonant interaction. By periodically deflecting the electron beam of a scanning electron microscope in close proximity to a spin-active solid-state sample, and sweeping the deflection frequency across the spin resonance, we directly observe phase coherent coupling between the electron beam's nearfield and the two spin states. This method relies only on classically shaping the electron beams transversal correlations and has the potential to enable coherent control of quantum systems with unprecedented, electron microscopic resolution, opening novel possibilities for advanced spectroscopic tools in nanotechnology.

Thermally induced fluctuations impose a fundamental limit on precision measurement. In optical interferometry, the current bounds of stability and sensitivity are dictated by the excess mechanical damping of the high-reflectivity coatings that comprise the cavity end mirrors. Over the preceding decade, the mechanical loss of these amorphous multilayer reflectors has at best been reduced by a factor of two. Here we demonstrate a new paradigm in optical coating technology based on direct-bonded monocrystalline multilayers, which exhibit both intrinsically low mechanical loss and high optical quality. Employing these "crystalline coatings" as end mirrors in a Fabry-Pérot cavity, we obtain a finesse of 150,000. More importantly, at room temperature, we observe a thermally-limited noise floor consistent with a tenfold reduction in mechanical damping when compared with the best dielectric multilayers. These results pave the way for the next generation of ultra-sensitive interferometers, as well as for new levels of laser stability.

Solid-state $^{229}$Th nuclear clocks are set to provide new opportunities for precision metrology and fundamental physics. Taking advantage of a nuclear transition's inherent low sensitivity to its environment, orders of magnitude more emitters can be hosted in a solid-state crystal compared to current optical lattice atomic clocks. Furthermore, solid-state systems needing only simple thermal control are key to the development of field-deployable compact clocks. In this work, we explore and characterize the frequency reproducibility of the $^{229}$Th:CaF$_2$ nuclear clock transition, a key performance metric for all clocks. We measure the transition linewidth and center frequency as a function of the doping concentration, temperature, and time. We report the concentration-dependent inhomogeneous linewidth of the nuclear transition, limited by the intrinsic host crystal properties. We determine an optimal working temperature for the $^{229}$Th:CaF$_2$ nuclear clock at 195(5) K where the first-order thermal sensitivity vanishes. This would enable in-situ temperature co-sensing using different quadrupole-split lines, reducing the temperature-induced systematic shift below the 10$^{-18}$ fractional frequency uncertainty level. At 195 K, the reproducibility of the nuclear transition frequency is 280 Hz (fractionally $1.4\times10^{-13}$) for two differently doped $^{229}$Th:CaF$_2$ crystals over four months. These results form the foundation for understanding, controlling, and harnessing the coherent nuclear excitation of $^{229}$Th in solid-state hosts, and for their applications in constraining temporal variations of fundamental constants.

We present a systematic derivation of the dynamical polarizability and the ac Stark shift of the ground and excited states of atoms interacting with a far-off-resonance light field of arbitrary polarization. We calculate the scalar, vector, and tensor polarizabilities of atomic cesium using resonance wavelengths and reduced matrix elements for a large number of transitions. We analyze the properties of the fictitious magnetic field produced by the vector polarizability in conjunction with the ellipticity of the polarization of the light field.

We study a setup where a single negatively-charged silicon-vacancy center in diamond is magnetically coupled to a low-frequency mechanical bending mode and via strain to the high-frequency phonon continuum of a semi-clamped diamond beam. We show that under appropriate microwave driving conditions, this setup can be used to induce a laser cooling like effect for the low-frequency mechanical vibrations, where the high-frequency longitudinal compression modes of the beam serve as an intrinsic low-temperature reservoir. We evaluate the experimental conditions under which cooling close to the quantum ground state can be achieved and describe an extended scheme for the preparation of a stationary entangled state between two mechanical modes. By relying on intrinsic properties of the mechanical beam only, this approach offers an interesting alternative for quantum manipulation schemes of mechanical systems, where otherwise efficient optomechanical interactions are not available.